A precision mass investigation of the neutron-rich titanium isotopes 51−55 Ti was performed at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The range of the measurements covers the N = 32 shell closure and the overall uncertainties of the 52−55 Ti mass values were significantly reduced. Our results conclusively establish the existence of weak shell effect at N = 32, narrowing down the abrupt onset of this shell closure. Our data were compared with state-of-the-art ab initio shell model calculations which, despite very successfully describing where the N = 32 shell gap is strong, overpredict its strength and extent in titanium and heavier isotones. These measurements also represent the first scientific results of TITAN using the newly commissioned Multiple-Reflection Time-of-Flight Mass Spectrometer (MR-TOF-MS), substantiated by independent measurements from TITAN's Penning trap mass spectrometer.Atomic nuclei are highly complex quantum objects made of protons and neutrons. Despite the arduous efforts needed to disentangle specific effects from their many-body nature, the fine understanding of their structures provides key information to our knowledge of fundamental nuclear forces. One notable quantum behavior of bound nuclear matter is the formation of shell-like structures for each fermion group [1], as electrons do in atoms. Unlike for atomic shells, however, nuclear shells are known to vanish or move altogether as the number of protons or neutrons in the system changes [2]. Particular attention has been given to the emergence of strong shell effects among nuclides with 32 neutrons, pictured in a shell model framework as a full valence ν2p 3/2 orbital. Across most of the known nuclear chart, this orbital is energetically close to ν1f 5/2 , which prevents the appearance of shell signatures in energy observables. However, the excitation energies of the lowest 2 + states show a relative, but systematic, local increase below proton number Z = 24 [3]. This effect, characteristic of shell closures, has been attributed in shell model calculations to the weakening of attractive proton-neutron interactions between the ν1f 5/2 and π1f 7/2 orbitals as the latter empties, making the neutrons in the former orbital less bound [4,5]. Ab initio calculations are also extending their reach over this sector of the nuclear chart, yet no systematic investigation of the N = 32 isotones has been produced so far.

Electrical breakdown and water surface deformation in a metal pin–water electrode system with dc applied voltages is studied for small inter-electrode distances (2–12 mm). The radius of curvature of the metal pin is 0.5 cm to exclude corona before breakdown at these small inter-electrode spacings. Calculations of the water surface deformation as a function of the applied voltage and initial inter-electrode spacing are compared with measurements of the water elevation. For distances smaller than 7 mm the calculated stability limit of the water surface corresponds with the experimentally obtained breakdown voltage. It is proved with fast CCD images and calculations of the electrical field distribution that the water surface instability triggers the electrical breakdown in this case. The images show that at breakdown the water surface has a Taylor cone-like shape. At inter-electrode distance of 7 mm and larger the breakdown voltage is well below the water stability limit and the conductive channel at breakdown is formed between the pin electrode and the static water surface. Both cases are discussed and compared.

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H+3 is the simplest triatomic molecule and plays an important role in laboratory and astrophysical plasmas. It is very stable both in terms of its electronic and nuclear degrees of freedom but is difficult to study in depth in the laboratory due to its ionic nature. In this communication, experimental results are presented for the strong field dissociation of the isotopic analogue D+3, using 30 fs, 800 nm laser pulses with intensities up to 1016 W cm−2. By employing a novel experimental set-up, ions were confined in an electrostatic ion trap so that dissociation of the molecule could be studied as it radiatively cools. It was determined that dissociation could only be observed for molecules in ro-vibrational states relatively close to the dissociation limit, while more tightly bound states demonstrated remarkable stability in even the strongest fields.

We performed the first direct mass measurements of neutron-rich vanadium 52−55 V isotopes passing the N = 32 neutron shell closure with TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The new direct measurements confirm all previous indirect results. Through a reduced uncertainty of the mass of 55 V we confirm the quenching of the N = 32 neutron shell closure in vanadium. We discuss the evolution of the N = 32 neutron shell closure between K and Cr and show similar signatures in the half-life surface when studied along the isotopic chains.

We demonstrate single-beam coherent anti-Stokes Raman spectroscopy (CARS), for detecting and identifying traces of solids, including minute amounts of explosives, from a standoff distance (>50 m) using intense femtosecond pulses. Until now, single-beam CARS methods relied on pulse-shapers in order to obtain vibrational spectra. Here we present a simple and easy-to-implement detection scheme, using a commercially available notch filter, that does not require the use of a pulse-shaper.

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We demonstrate the ability to control the molecular dissociation rate using femtosecond pulses shaped with third-order dispersion (TOD). Explicitly, a significant 50% enhancement in the dissociation yield for the low lying vibrational levels (v ∼ 6) of an ion-beam target was measured as a function of TOD. The underlying mechanism responsible for this enhanced dissociation was theoretically identified as non-adiabatic alignment induced by the pre-pulses situated on the leading edge of pulses shaped with negative TOD. This control scheme is expected to work in other molecules as it does not rely on specific characteristics of our test-case molecule.