Nuclear reactions where an exotic nucleus captures a neutron are critical for a wide variety of applications, from energy production and national security, to astrophysical processes, and nucleosynthesis. Neutron capture rates are well constrained near stable isotopes where experimental data are available; however, moving far from the valley of stability, uncertainties grow by orders of magnitude. This is due to the complete lack of experimental constraints, as the direct measurement of a neutron-capture reaction on a short-lived nucleus is extremely challenging. Here, we report on the first experimental extraction of a neutron capture reaction rate on ^{69}Ni, a nucleus that is five neutrons away from the last stable isotope of Ni. The implications of this measurement on nucleosynthesis around mass 70 are discussed, and the impact of similar future measurements on the understanding of the origin of the heavy elements in the cosmos is presented.
Nuclear level densities and γ-ray strength functions of 56,57Fe have been extracted from proton-γ coincidences. A low-energy enhancement in the γ-ray strength functions up to a factor of 30 over common theoretical E1 models is confirmed. Angular distributions of the low-energy enhancement in 57Fe indicate its dipole nature, in agreement with findings for 56Fe. The high statistics and the excellent energy resolution of the large-volume LaBr3(Ce) detectors allowed for a thorough analysis of γ strength as function of excitation energy. Taking into account the presence of strong Porter–Thomas fluctuations, there is no indication of any significant excitation energy dependence in the γ-ray strength function, in support of the generalized Brink–Axel hypothesis.
Particle-γ coincidence data have been analyzed to obtain the nuclear level density and the γ -strength function of 64 Ni by means of the Oslo method. The level density found in this work is in very good agreement with known energy levels at low excitation energies as well as with data deduced from particle-evaporation measurements at excitation energies above E x ≈ 5.5 MeV. The experimental γ -strength function presents an enhancement at γ energies below E γ ≈ 3 MeV and possibly a resonancelike structure centered at E γ ≈ 9.2 MeV. The obtained nuclear level density and γ -strength function have been used to estimate the (n,γ ) cross section for the s-process branch-point nucleus 63 Ni, of particular interest for astrophysical calculations of elemental abundances.
Neutron-capture reactions on very neutron-rich nuclei are essential for heavy-element nucleosynthesis through the rapid neutron-capture process, now shown to take place in neutron-star merger events. For these exotic nuclei, radiative neutron capture is extremely sensitive to their γ-emission probability at very low γ energies. In this work, we present measurements of the γ-decay strength of 70 Ni over the wide range 1.3 ≤ E γ ≤ 8 MeV. A significant enhancement is found in the γ-decay strength for transitions with E γ < 3 MeV. At present, this is the most neutron-rich nucleus displaying this feature, proving that this phenomenon is not restricted to stable nuclei. We have performed E1-strength calculations within the quasiparticle time-blocking approximation, which describe our data above E γ 5 MeV very well. Moreover, large-scale shell-model calculations indicate an M1 nature of the low-energy γ strength. This turns out to be remarkably robust with respect to the choice of interaction, truncation and model space, and we predict its presence in the whole isotopic chain, in particular the neutron-rich 72,74,76 Ni.
The effect of both a RF sputtered Al-doped ZnO (AZO) thin film seed layer onto a FTO/glass substrate and its growth time onto the morphological, structural and optical properties of the resulting electrochemically grown ZnO nanorod arrays (NRAs) have been studied. ZnO NRs grown onto the different AZO seed layers exhibit smaller mean diameter and length than those grown onto a bare FTO/glass substrate, but ZnO NR density presents an opposite behavior, by using an AZO seed layer ZnO nanorod density can be increased by a factor of six. ZnO nanorods are highly crystalline with a wurtzite hexagonal structure and with a preferential growth perpendicular to the substrate. The c-axis of most of the ZnO NRs grown onto an AZO seed layer is aligned within ±6 • from the substrate surface normal. Both NRAs mean length and density increases light scattering, without greatly affecting the spectra shape. The diffuse reflectance intensity is more sensitive to NR density variations than to length or diameter variations. NR diameter affects directly the shape of these diffuse reflectance spectra: they red-shifts and broadens when NR mean diameter increases. A small influence in the UV edge due to size quantization may be also present. In recent years, ZnO, a wide bandgap semiconductor with a direct bandgap of about 3.37 eV and high exciton binding energy (60 meV) at room temperature, has attracted increasing interest due to its unique ability to form a variety of nanostructures such as nanowires, nanorods, nanobelts, nanocombs, nanospheres, nano-tetrapods.1,2 Among them, the most interesting are nanorods and nanorod arrays (NRAs) vertically arranged with respect to the substrate.1 These ZnO nanostructures present a pseudo-one dimensional (1D) structure, with an enhanced surface-to-volume ratio and confinement effects.3 ZnO nanorods exhibit fewer defects than its thin-film structure, it is, therefore, a promising material for optoelectronic applications. 4 In fact, recently, single crystal ZnO nanowire and nanorod arrays have emerged as promising building blocks for a new generation of devices in different hi-tech domains such as optoelectronics, gas sensing, field emission, piezoelectrics and solar cells. 2,5,6 In particular, ZnO one dimensional nanostructures are good candidates for photovoltaic applications for three straightforward reasons: i) they have a low reflectivity that enhances the light absorption; ii) relatively high surface to volume ratio that enables interfacial charge separation and iii) fast electron transport along the crystalline 1D nanostructures that improves the charge collection efficiency. In fact, ZnO arrays of 1D nanostructures, such as nanowires and nanotubes, have been widely utilized as they provide a direct conduction pathway for the rapid collection of the photogenerated electrons, 7 reducing the non-radiative recombination and carrier scattering loss dramatically, 8 and providing as well a high junction area.9,10 Moreover, electron transport in the crystalline nanorod is expected to be several orde...
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