6,13-bis(triisopropylsilylethynyl) pentacene (TIPS pentacene) from simple drop casting typically forms crystals with random orientation and poor areal coverage, which leads to device-to-device performance variation of organic thin film transistors (OTFTs). Previously, a temperature gradient technique was developed to address these problems. However, this approach simultaneously introduced thermal cracks due to the thermally induced stress during crystallization. These thermal cracks accounted for a reduction of charge transport, thereby impacting the device performance of TIPS pentacene based OTFTs. In this work, an insulating polymer, poly(α-methyl styrene) (PαMS) was blended with TIPS pentacene to relieve the thermal stress and effectively prevent the generation of thermal cracks. The results demonstrate that the incorporation of PαMS polymer combined with the temperature gradient technique improves both the hole mobility and performance consistency of TIPS pentacene based OTFTs.
The utilization of three-dimensional (3D) structures in next-generation nanodevices has been attractive due to the exceptional features they offer. These 3D structures can reduce component space and improve device properties compared to thin-film electronic components. The type of transistor applied in 3D nanodevices is one of the most widely studied components due to its rich physics and ubiquitous application. In this paper, we report a complete functionalized component, a 3D vertical resonant photo-effect-transistor (VRPET), which is realized with the functionalized nanowire current channel, asymmetric ohmic/Schottky contacts, and an ultraviolet photogate with an organic light emission diode (OLED) excitation. To enhance the VRPET performance, analyses of the design and fabrication parameters were carried out, where the focus was specifically on the relationship between light resonance and absorption. The transistor developed here can operate up to a high voltage of 16.5 V and control currents up to 50 μA with an ultrastable performance under a strong electromagnetic interference. The VRPET with excellent properties is a step toward achieving integrated photoelectric devices and corresponding applications.
Phototriggered devices have attracted attention due to their exceptional characteristics, advanced multifunctionalities and unprecedented applications in optoelectronic systems. Here, we report a pioneer structural device, a resonant photoeffect-transistor (RPET) with a functionalized nanowire (NW) charge transport channel, modulated by a near-field nanostrip organic light emitting diode (OLED) and controlled by a gate bias to realize exceptional photoelectric properties. The RPET presents high-quality nanowire channel characteristics due to tunable optical cavities manifesting strong standing wave resonance under controlled light emission. To enhance performance, methodical analyses were carried out to determine the effects of the structural design, electric field distribution and charge carrier generation on photoresponsivity when light traverses a single or multiple nanoslit masks. The developed RPET yields stable photocurrents in the 10 5 range and generates current on/off ratios upward of 10 6 under the influence of intense electromagnetic distribution, effectively lending itself to promising opportunities in fully integrated optoelectronic devices.
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