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Peak and average power scalability is the key feature of advancing femtosecond laser technology. Today, near-infrared light sources are capable of providing hundreds of Watts of average power. These sources, however, scarcely deliver pulses shorter than 100 fs which are, for instance, highly beneficial for frequency conversion to the extreme ultraviolet or to the mid- infrared. Therefore, the development of power scalable pulse compression schemes is still an ongoing quest. This article presents the compression of 90 W average power, 190 fs pulses to 70 W, 30 fs. An increase in peak power from 18 MW to 60 MW is achieved. The compression scheme is based on cascaded phase-mismatched quadratic nonlinearities in BBO crystals. In addition to the experimental results, simulations are presented which compare spatially resolved spectra of pulses spectrally broadened in self-focusing and self-defocusing media, respectively. It is demonstrated that balancing self- defocusing and Gaussian beam convergence results in an efficient, power-scalable spectral broadening mechanism in bulk material.

We present a mid-infrared (MIR) source based on intrapulse difference-frequency generation under the random quasi-phase-matching condition. The scheme enables the use of non-birefringent materials whose crystal orientations are not perfectly and periodically poled, widening the choice of media for nonlinear frequency conversion. With a 2 μm driving source based on a Ho:YAG thin-disk laser, together with a polycrystalline ZnSe element, an octavespanning MIR continuum (2.7-20 μm) was generated. At over 20 mW, the average power is comparable to regular phase-matching in birefringent crystals. A 1 μm laser system based on a Yb:YAG thin-disk laser was also tested as a driving source in this scheme. The new approach provides a simplified way for generating coherent MIR radiation with an ultrabroad bandwidth at reasonable efficiency.

We present directly oscillator-driven self-compression inside an all-bulk Herriott-type multi-pass cell in the near-infrared spectral range. By utilizing precise dispersion management of the multi-pass cell mirrors, we achieve pulse compression from 300 fs down to 31 fs at 11 µJ pulse energy and 119 W average power with a total efficiency exceeding 85%. This corresponds to an increase in peak power by more than a factor of three and a temporal compression by almost a factor of ten in a single broadening stage without necessitating subsequent dispersive optics for temporal compression. The concept is scalable towards millijoule pulse energies and can be implemented in visible, near-infrared and infrared spectral ranges. Importantly, it paves a way towards exploiting Raman soliton self-frequency shifting, supercontinuum generation and other highly nonlinear effects at unprecedented high peak power and pulse energy levels.