We report the synthesis of (Ca₀.₃₃Na₀.₆₆)Fe₂As₂ showing a superconducting transition with T(c) above 33 K. Both dc magnetic susceptibility or specific heat measurements indicated the bulk superconductivity nature of the sample. We also have successfully grown single crystals of the (Ca₀.₃₃Na₀.₆₆)Fe₂As₂ superconductors. The single crystals exhibit sharp superconducting transitions with T(c) above 33 K. The effects of magnetic field on the superconducting transitions are studied, giving rise to high upper critical fields with H(c₂)(c)≈85 T and H(c₂)(ab)≈172 T, respectively. The anisotropy parameter was calculated to be around 2.
To explore the origin of the unusual non-bulk superconductivity with a T c up to 49 K reported in the rareearth-doped CaFe 2 As 2 , the chemical composition, magnetization, specific heat, resistivity, and annealing effect are systematically investigated on nominal (Ca 1-x R x )Fe 2 As 2 single crystals with different x's and R = La, Ce, Pr, and Nd. All display a doping-independent T c once superconductivity is induced, a doping-dependent low field superconducting volume fraction f, and a large magnetic anisotropy η in the superconducting state, suggesting a rather inhomogeneous superconducting state in an otherwise microscale-homogenous superconductor. The wavelength dispersive spectroscopy and specific heat show the presence of defects which are closely related to f, regardless of the R involved. The magnetism further reveals that the defects are mainly superparamagnetic clusters for R = Ce, Pr, and Nd with strong intercluster interactions, implying that defects are locally self-organized. Annealing at 500 °C, without varying the doping level x, suppresses f profoundly but not the T c . The above observations provide evidence for the crucial role of defects in the occurrence of the unusually high T c ~ 49 K in (Ca 1-x R x )Fe 2 As 2 and are consistent with the interface-enhanced superconductivity recently proposed.
We report the anomalous Hall effect (AHE) in antiperovskite Mn3NiN with substantial doping of Cu on the Ni site (i.e. Mn3Ni1−xCuxN), which stabilizes a noncollinear antiferromagnetic (AFM) order compatible with the AHE. Observed on both sintered polycrystalline pieces and single crystalline films, the AHE does not scale with the net magnetization, contrary to the conventional ferromagnetic case. The existence of the AHE is explained through symmetry analysis based on the Γ4g AFM order in Cu doped Mn3NiN. DFT calculations of the intrinsic contribution to the AHE reveal the non-vanishing Berry curvature in momentum space due to the noncollinear magnetic order. Combined with other attractive properties, antiperovskite Mn3AN system offers great potential in AFM spintronics.
Spin ices are exotic phases of matter characterized by frustrated spins obeying local "ice rules", in analogy with the electric dipoles in water ice. In two dimensions, one can similarly define ice rules for in-plane Ising-like spins arranged on a kagome lattice. These ice rules require each triangle plaquette to have a single monopole, and can lead to various unique orders and excitations. Using experimental and theoretical approaches including magnetometry, thermodynamic measurements, neutron scattering and Monte Carlo simulations, we establish HoAgGe as a crystalline (i.e. non-artificial) system that realizes the kagome spin ice state. The system features a variety of partially and fully ordered states and a sequence of field-induced phases at low temperatures, all consistent with the kagome ice rule.
We have synthesized single crystals of Dirac semimetal candidates AZnBi2 with A=Ba and Sr. In contrast to A=Sr, the Ba material displays a novel local Zn vacancy ordering, which makes the observation of quantum oscillations in out-of-plane magnetic fields possible. As a new Dirac semimetal candidate, BaZnBi2 exhibits small cyclotron electron mass, high quantum mobility, and non-trivial Berry phases. Three Dirac dispersions are observed by ARPES and identified by firstprinciples band-structure calculations. Compared to AMn(Bi/Sb)2 systems which host Mn magnetic moments, BaZnBi2 acts as non-magnetic analogue to investigate the intrinsic properties of Dirac fermions in this structure family.
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