Synchronous laser-microwave networks delivering attosecond timing precision are highly desirable in many advanced applications, such as geodesy, very-long-baseline interferometry, high-precision navigation and multi-telescope arrays. In particular, rapidly expanding photon-science facilities like X-ray free-electron lasers and intense laser beamlines require system-wide attosecond-level synchronization of dozens of optical and microwave signals up to kilometer distances. Once equipped with such precision, these facilities will initiate radically new science by shedding light on molecular and atomic processes happening on the attosecond timescale, such as intramolecular charge transfer, Auger processes and their impacts on X-ray imaging. Here we present for the first time a complete synchronous laser-microwave network with attosecond precision, which is achieved through new metrological devices and careful balancing of fiber nonlinearities and fundamental noise contributions. We demonstrate timing stabilization of a 4.7-km fiber network and remote optical–optical synchronization across a 3.5-km fiber link with an overall timing jitter of 580 and 680 attoseconds root-mean-square, respectively, for over 40 h. Ultimately, we realize a complete laser-microwave network with 950-attosecond timing jitter for 18 h. This work can enable next-generation attosecond photon-science facilities to revolutionize many research fields from structural biology to material science and chemistry to fundamental physics.

Coherently-pumped (Kerr) solitons in an ideal optical microcavity are expected to undergo random quantum motion that determines fundamental performance limits in applications of soliton microcombs. Here, this diffusive motion and its impact on Kerr soliton timing jitter is studied experimentally. Typically hidden below technical noise contributions, the quantum limit is discerned by measuring counter-propagating solitons. Their relative motion features only weak interactions and also presents excellent common mode suppression of technical noise. This is in strong contrast to co-propagating solitons which are found to have relative timing jitter well below the quantum limit of a single soliton on account of strong mutual motion correlation. Good agreement is found between theory and experiment. The results establish the fundamental limits to timing jitter in soliton microcombs and provide new insights on multi-soliton physics.Recently, coherently pumped solitons 1,2 have been realized in optical microcavities 3 . Unlike earlier temporal optical solitons, these new solitons are able to regenerate through Kerr-induced parametric amplification 4,5 , and strong resonant build-up in the high-Q microcavity enables access to optical nonlinearity at low power levels 6 .

Ultra-precise timing has become a prerequisite for many modern large-scale scientific instruments, and timing precision is a crucial enabling factor to achieve the ultimate goals of those instruments. Here, we review the recent progress in timing technologies, including timing characterization methods among different kinds of sources (optical lasers, microwaves and x-ray pulses), large-scale free-space timing synchronization, and fiber-based timing synchronization. Technical and fundamental limitations of fiber-based timing systems are also discussed to provide future directions.

In this Letter, we investigate steady states of fiber lasers mode-locked with a nonlinear amplifying loop mirror that have an inherent amplitude-noise-suppression mechanism. Due to the interaction of the sinusoidal transmission function with the fluctuating intracavity pulse amplitude, we show that under specific preconditions, this mechanism may lead to a detectable difference in relative intensity noise at the reflected and transmitted output port of the laser. We present systematic intensity noise measurements with a nonlinear fiber-based system that replicates a single roundtrip in the laser cavity. The experimental results and simulations clearly show a reduction of the intracavity amplitude fluctuations up to 4 dB for certain steady states.