Optically pumped mirrorless laser action has been observed in a dye-doped flexible free-standing film of photopolymerized cholesteric liquid crystal (PCLC). In the PCLC film, self-organized helical structure acts as one-dimensional (1D) photonic crystal. At high excitation intensity above the threshold, a laser action is observed at an edge of the 1D photonic band of the PCLC helical structure. This PCLC film laser possesses an excellent mechanical flexibility, and the laser action is also observed in a bent film of PCLC. This implies that the one-dimensional periodic structure for the laser action is maintained even in the deformed film. Using such flexibility of the PCLC film, a focusing effect of laser emission is demonstrated in a circularly deformed film. Moreover, the helical pitch of the PCLC has no temperature dependence in contrast to that of unpolymerized cholesteric liquid crystal. This means that the operation wavelength of laser action is thermally stable, which is the great advantage for the device application.
Various types of tunable lasing in dye-doped liquid crystals with one dimensional periodic structure have been demonstrated. An electrical tuning of lasing wavelength has been demonstrated in a dye-doped chiral smectic liquid crystal mixture with a short pitch helical structure which is so-called ferroelectric liquid crystal (FLC). Waveguide configuration of FLC laser has also been proposed. also in which the lasing wavelength widely can be tuned upon the electric filed. The electrically tunable lasing has been observed also in a focal conic structure of dye-doped cholesteric liquid crystal. This laser action is based on a helix micro-cavity in focal conic domains. Optically pumped distributed feedback lasing has been proposed in a dye-doped nematic liquid crystal (NLC) waveguide by holographic excitation. in which continuous tuning of the lasing wavelength is performed upon applying electric filed. Electrical tuning of the wavelength of the defect mode lasing in a one-dimensional periodic structure has been demonstrated using a dye-doped NLC as a defect layer in the periodic structure. Lasing wavelength is widely tuned upon applying the electric field. which is due to the refractive index change in the defect layer caused by the field-induced realignment of the NLC molecules.
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