Laser excitation of nanometer-sized atomic and molecular clusters offers
various opportunities to explore and control ultrafast many-particle dynamics.
Whereas weak laser fields allow the analysis of photoionization, excited-state
relaxation, and structural modifications on these finite quantum systems,
large-amplitude collective electron motion and Coulomb explosion can be induced
with intense laser pulses. This review provides an overview of key phenomena
arising from laser-cluster interactions with focus on nonlinear optical
excitations and discusses the underlying processes according to the current
understanding. A brief general survey covers basic cluster properties and
excitation mechanisms relevant for laser-driven cluster dynamics. Then, after
an excursion in theoretical and experimental methods, results for single- and
multiphoton excitations are reviewed with emphasis on signatures from time- and
angular resolved photoemission. A key issue of this review is the broad
spectrum of phenomena arising from clusters exposed to strong fields, where the
interaction with the laser pulse creates short-lived and dense nanoplasmas. The
implications for technical developments include the controlled generation of
ion, electron, and radiation pulses, as will be addressed along with
corresponding examples. Finally, future prospects of laser-cluster research as
well as experimental and theoretical challenges are discussed.Comment: text and figures revise
The current paper presents a state-of-the-art review in the field of interaction of atomic and molecular clusters with solids. We do not attempt to overview the entire broad field, but rather concentrate on the impact phenomena: how the physics of the cluster-surface interaction depends on the kinetic energy and what effects are induced under different energetic regimes. The review starts with an introduction to the field and a short history of cluster beam development. Then fundamental physical aspects of cluster formation and the most common methods for the production of cluster beams are overviewed. For cluster-surface interactions, one of the important scenarios is the low-energy regime where the kinetic energy per atom of the accelerated cluster stays well below the binding (cohesive) energy of the cluster constituents. This case is often called This is the peer-reviewed author's version of a work that was accepted for publication in Surface Science Reports. Changes resulting from the publishing process, such as editing, corrections, structural formatting, and other quality control mechanisms may not be reflected in this document. Changes may have been made to this work since it was submitted for publication. A definitive version
The interaction of intense extreme ultraviolet femtosecond laser pulses ( 32:8 nm) from the FLASH free electron laser (FEL) with clusters has been investigated by means of photoelectron spectroscopy and modeled by Monte Carlo simulations. For laser intensities up to 5 10 13 W=cm 2 , we find that the cluster ionization process is a sequence of direct electron emission events in a developing Coulomb field. A nanoplasma is formed only at the highest investigated power densities where ionization is frustrated due to the deep cluster potential. In contrast with earlier studies in the IR and vacuum ultraviolet spectral regime, we find no evidence for electron emission from plasma heating processes.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.