Cellulose has been discovered as a smart material that can be used as sensor and actuator material. In this paper, cellulose smart material termed as electro-active paper (EAPap) is prepared by an automated process that includes tape casting and zone stretching. To evaluate characteristics of the EAPap, its Young's modulus and piezoelectric charge constant are measured depending on the orientation angle, in comparison with the manually fabricated EAPap results. The zone stretching method can effectively align the cellulose fibers in the EAPap so as to improve its Young's modulus as well as piezoelectric charge constant. The 0 degree oriented sample shows its maximum Young's modulus and the 45 degree oriented sample exhibits the maximum piezoelectric charge constant. This 45 degree is associated with its shear piezoelectricity. The actuator performance of EAPap is evaluated by measuring its bending displacement depending on the orientation angle and the excitation voltage. The 45 degree oriented sample exhibits the maximum bending displacement. Details of the material preparation, the automation process, characterization and the actuator performance are addressed. This automated process that includes tape casting and zone stretching is suitable for mass production of the EAPap.
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