We report on the observation of cyclotron resonance induced photocurrents, excited by continuous wave terahertz radiation, in a 3D topological insulator (TI) based on an 80 nm strained HgTe film. The analysis of the photocurrent formation is supported by complimentary measurements of magneto-transport and radiation transmission. We demonstrate that the photocurrent is generated in the topologically protected surface states. Studying the resonance response in a gated sample we examined the behavior of the photocurrent, which enables us to extract the mobility and the cyclotron mass as a function of the Fermi energy. For high gate voltages we also detected cyclotron resonance (CR) of bulk carriers, with a mass about two times larger than that obtained for the surface states. The origin of the CR assisted photocurrent is discussed in terms of asymmetric scattering of TI surface carriers in the momentum space. Furthermore, we show that studying the photocurrent in gated samples provides a sensitive method to probe the effective masses and the mobility of 2D Dirac surface states, when the Fermi level lies in the bulk energy gap or even in the conduction band.
We report on the observation of the giant photocurrents in HgTe/HgCdTe quantum well (QW) of critical thickness at which a Dirac spectrum emerges. At an exciting QW of 6.6 nm width by terahertz (THz) radiation and sweeping magnetic field we detected a resonant photocurrent. Remarkably, the position of the resonance can be tuned from negative (−0.4 T) to positive (up to 1.2 T) magnetic fields by means of optical doping. The photocurrent data, accompanied by measurements of radiation transmission as well as Shubnikov-de Haas and quantum Hall effects, prove that the photocurrent is caused by cyclotron resonance in a Dirac fermion system, which allows us to obtain the effective electron velocity v ≈ 7.2 × 10 5 m/s. We develop a microscopic theory of the effect and show that the inherent spin-dependent asymmetry of light-matter coupling in the system of Dirac fermions causes the electric current to flow.
We report on the observation of a circular photogalvanic current excited by terahertz laser radiation in helical edge channels of two-dimensional (2D) HgTe topological insulators (TIs). The direction of the photocurrent reverses by switching the radiation polarization from a right-handed to a left-handed one and, for fixed photon helicity, is opposite for the opposite edges. The photocurrent is detected in a wide range of gate voltages. With decreasing the Fermi level below the conduction band bottom, the current emerges, reaches a maximum, decreases, changes its sign close to the charge neutrality point (CNP), and again rises. Conductance measured over a ≈3 μm distance at CNP approaches 2e 2 /h, the value characteristic for ballistic transport in 2D TIs. The data reveal that the photocurrent is caused by photoionization of helical edge electrons to the conduction band. We discuss the microscopic model of this phenomenon and compare calculations with experimental data. DOI: 10.1103/PhysRevB.95.201103 The quantum spin Hall (QSH) effect occurs in 2D TIs and rests on the existence of conducting helical edge states while the bulk is insulating [1][2][3][4]. In contrast to the quantum Hall effect, the formation of these edge states requires no magnetic field: they stem from the band inversion caused by strong spin-orbit interaction and are topologically protected by time reversal symmetry. Given that the spin-up and spin-down electrons propagate along an edge in opposite directions, i.e., the spin projection is locked to the k vector, the edge channels are helical in nature. The first experimental evidence for the QSH effect was obtained in HgTe quantum wells (QWs) [5] by observing a resistance plateau around h/2e 2 in the longitudinal resistance of a mesoscopic Hall bar. Here h is Planck's constant and e is the electron charge. This observation was further confirmed by nonlocal experiments in the ballistic [6] and diffusive [7] transport regime. Conducting edge channels were later probed by scanning SQUID microscopy [8], scanning gate microscopy [9], microwave impedance microscopy [10], and by analyzing supercurrents [11]. The spin polarization of the edge states was investigated so far by electrical means only: by detecting the spin to charge conversion in devices utilizing the inverse spin Hall effect [12] or with ferromagnetic contacts [13].Here we use circularly polarized terahertz radiation to excite selectively spin-up and spin-down electrons circling clockwise and counterclockwise around a sample. We show that the excitation causes an imbalance in the electron distribution between positive and negative wave vectors. This is probed as the associated photogalvanic [14,15] current, which reverses its direction upon switching the helicity.The experiments have been carried out on Hg 0.3 Cd 0.7 Te/HgTe/Hg 0.3 Cd 0.7 Te single QW structures with a well width of 8 nm having inverted band ordering. We used this width to maximize the energy gap to about 25 meV [4,5]. Structures were grown by molecular beam epitaxy o...
We report on the observation of magneto-oscillations of terahertz radiation induced photocurrent in HgTe/HgCdTe quantum wells of different widths, which are characterized by a Dirac-like, inverted, and normal parabolic band structure. The photocurrent data are accompanied by measurements of photoresistance (photoconductivity), radiation transmission, as well as magnetotransport. We develop a microscopic model of a cyclotron-resonance assisted photogalvanic effect, which describes main experimental findings. We demonstrate that the quantum oscillations of the photocurrent are caused by the crossing of Fermi level by Landau levels resulting in the oscillations of spin polarization and electron mobilities in spin subbands. Theory explains a photocurrent direction reversal with the variation of magnetic field observed in experiment. We describe the photoconductivity oscillations related with the thermal suppression of the Shubnikov-de Haas effect.
We report on the observation of the giant photocurrent in HgTe/HgCdTe quantum wells (QW) of critical thickness at which a Dirac spectrum emerges 1 , 2 . Exciting QW of 6.6 nm width by terahertz (THz) radiation and sweeping the magnetic field we detected a resonant photocurrent. Remarkably, the position of the resonance can be tuned from negative (-0.4 T) to positive (up to 1.2 T) magnetic fields by means of optical doping. We show that the photocurrent is caused by cyclotron resonance (CR) in a Dirac fermion system, which allows us to obtain the electron velocity v -7.2 10 5 m/s. We develop a microscopic theory of the effect and show that the inherent spin dependent asymmetry of the Dirac fermion scattering in QWs causes the electric current to flow.
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