[1] The paper presents the current status of the Maritime Aerosol Network (MAN), which has been developed as a component of the Aerosol Robotic Network (AERONET). MAN deploys Microtops handheld Sun photometers and utilizes the calibration procedure and data processing (Version 2) traceable to AERONET. A web site dedicated to the MAN activity is described. A brief historical perspective is given to aerosol optical depth (AOD) measurements over the oceans. A short summary of the existing data, collected on board ships of opportunity during the NASA Sensor Intercomparison and Merger for Biological and Interdisciplinary Oceanic Studies (SIMBIOS) Project is presented. Globally averaged oceanic aerosol optical depth (derived from island-based AERONET measurements) at 500 nm is $0.11 and Angstrom parameter (computed within spectral range 440-870 nm) is calculated to be $0.6. First results from the cruises contributing to the Maritime Aerosol Network are shown. MAN ship-based aerosol optical depth compares well to simultaneous island and near-coastal AERONET site AOD.

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[1] The Indo-Gangetic Plain (IGP) encompasses a vast area, (accounting for $21% of the land area of India), which is densely populated (accommodating $40% of the Indian population). Highly growing economy and population over this region results in a wide range of anthropogenic activities. A large number of thermal power plants (most of them coal fed) are clustered along this region. Despite its importance, detailed investigation of aerosols over this region is sparse. During an intense field campaign of winter 2004, extensive aerosol and atmospheric boundary layer measurements were made from three locations: Kharagpur (KGP), Allahabad (ALB), and Kanpur (KNP), within the IGP. These data are used (1) to understand the regional features of aerosols and BC over the IGP and their interdependencies, (2) to compare it with features at locations lying at far away from the IGP where the conditions are totally different, (3) to delineate the effects of mesoscale processes associated with changes in the local atmospheric boundary layer (ABL), (4) to investigate the effects of long-range transport or moving weather phenomena in modulating the aerosol properties as well as the ABL characteristics, and (5) to examine the changes as the season changes over to spring and summer. Our investigations have revealed very high concentrations of aerosols along the IGP, the average mass concentrations (M T ) of total aerosols being in the range 260 to 300 mg m À3 and BC mass concentrations (M B ) in the range 20 to 30 mg m À3 (both $5 to 8 times higher than the values observed at off-IGP stations) during December 2004. Despite, BC constituted about 10% to the total aerosol mass concentration, a value quite comparable to those observed elsewhere over India for this season. The dynamics of the local atmospheric boundary layer (ABL) as well as changes in local emissions strongly influence the diurnal variations of M T and M B , both being inversely correlated with the mixed layer height (Z i ) and the ventilation coefficient (V c ). The share of BC to total aerosols is highest ($12%) during early night and lowest ($4%) in the early morning hours. While an increase in the V c results in a reduction in the concentration almost simultaneously, an increase in Z imax has its most impact on the concentration after $1 day. Accumulation mode aerosols contributed $90% to the aerosol concentration at ALB, $77 % at KGP and 74% at KNP. The BC mass mixing ratio was $10% over all three locations and is comparable to the value reported for Trivandrum, a tropical coastal location in southern India. This indicates presence of submicron aerosols species other than BC (such as sulfate) over KGP and KNP. A cross-correlation analysis showed that the changes in M B at KGP is significantly correlated with those at KNP, located $850 km upwind, and ALB after a delay of $7 days, while no such delay was seen between ALB and KNP. Back trajectory analyses show an enhancement in M B associated with trajectories arriving from west, the farther from to the west they arr...

[1] The first regional synthesis of long-term (back to~25 years at some stations) primary data (from direct measurement) on aerosol optical depth from the ARFINET (network of aerosol observatories established under the Aerosol Radiative Forcing over India (ARFI) project of Indian Space Research Organization over Indian subcontinent) have revealed a statistically significant increasing trend with a significant seasonal variability. Examining the current values of turbidity coefficients with those reported~50 years ago reveals the phenomenal nature of the increase in aerosol loading. Seasonally, the rate of increase is consistently high during the dry months (December to March) over the entire region whereas the trends are rather inconsistent and weak during the premonsoon (April to May) and summer monsoon period (June to September). The trends in the spectral variation of aerosol optical depth (AOD) reveal the significance of anthropogenic activities on the increasing trend in AOD. Examining these with climate variables such as seasonal and regional rainfall, it is seen that the dry season depicts a decreasing trend in the total number of rainy days over the Indian region. The insignificant trend in AOD observed over the Indo-Gangetic Plain, a regional hot spot of aerosols, during the premonsoon and summer monsoon season is mainly attributed to the competing effects of dust transport and wet removal of aerosols by the monsoon rain. Contributions of different aerosol chemical species to the total dust, simulated using Goddard Chemistry Aerosol Radiation and Transport model over the ARFINET stations, showed an increasing trend for all the anthropogenic components and a decreasing trend for dust, consistent with the inference deduced from trend in Angstrom exponent.

[1] During a comprehensive aerosol field campaign, simultaneous measurements were made of aerosol spectral optical depths, black carbon mass concentration (M b ), total (M t ) and size segregated aerosol mass concentrations over an urban continental location, Bangalore (13°N, 77°E, 960 m msl), in India. Large amounts of BC were observed; both in absolute terms and fraction of total mass ($11%) and submicron mass ($23%) implying a significantly low single scatter albedo. The aerosol visible optical depth (t p ) was in the range 0.24 to 0.45. Estimated surface forcing is as high as À23 W m À2 and top of the atmosphere (TOA) forcing is +5 W m À2 during relatively cleaner periods (t p $ 0.24). The net atmospheric absorption translates to an atmospheric heating of $0.8 K day À1 for cleaner periods and $1.5 K day À1 for less cleaner periods (t p $ 0.45). Our observations raise several issues, which may have impacts to regional climate and monsoon.

[1] Extensive intercomparison of columnar and near-surface aerosols, simulated over the South Asian domain using the aerosol module included in the regional climate model (RegCM4) of the Abdus Salam International Centre for Theoretical Physics (ICTP) have been carried out using ground-based network of Sun/sky Aerosol Robotic Network (AERONET) radiometers, satellite sensors such as Moderate Resolution Imaging Spectroradiometer (MODIS) and Multiangle Imaging Spectroradiometer (MISR), and ground-based black carbon (BC) measurements made at Aerosol Radiative Forcing over India (ARFI) network stations. In general, RegCM4 simulations reproduced the spatial and seasonal characteristics of aerosol optical depth over South Asia reasonably well, particularly over west Asia, where mineral dust is a major contributor to the total aerosol loading. In contrast, RegCM4 simulations drastically underestimated the BC mass concentrations over most of the stations, by a factor of 2 to 5, with a large spatial variability. Seasonally, the discrepancy between the measured and simulated BC tended to be higher during winter and periods when the atmospheric boundary layer is convectively stable (such as nighttime and early mornings), while during summer season and during periods when the boundary layer is convectively unstable (daytime) the discrepancies were much lower, with the noontime values agreeing very closely with the observations. A detailed analysis revealed that the model does not reproduce the nocturnal high in BC, observed at most of the Indian sites especially during winter, because of the excessive vertical transport of aerosols under stable boundary layer conditions. As far as the vertical distribution was concerned, the simulated vertical profiles of BC agreed well with airborne measurements during daytime. This comprehensive validation exercise reveals the strengths and weaknesses of the model in simulating the spatial and temporal heterogeneities of the aerosol fields over South Asia.

Abstract. The Maritime Aerosol Network (MAN) has been collecting data over the oceans since November 2006. Over 80 cruises were completed through early 2010 with deployments continuing. Measurement areas included various parts of the Atlantic Ocean, the Northern and Southern Pacific Ocean, the South Indian Ocean, the Southern Ocean, the Arctic Ocean and inland seas. MAN deploys Microtops handheld sunphotometers and utilizes a calibration procedure and data processing traceable to AERONET. Data collection included areas that previously had no aerosol optical depth (AOD) coverage at all, particularly vast areas of the Southern Ocean. The MAN data archive provides a valuable resource for aerosol studies in maritime environments. In the current paper we present results of AOD measurements over the oceans, and make a comparison with satellite AOD retrievals and model simulations.

[1] Collocated measurements of the mass concentrations of aerosol black carbon (BC) and composite aerosols near the surface were carried out along with spectral aerosol optical depths (AODs) from a high-altitude station, Manora Peak in central Himalayas, during a comprehensive aerosol field campaign in December 2004. Despite being a pristine location in the Shivalik Ranges of central Himalayas and having a monthly mean AOD (at 500 nm) of 0.059 ± 0.033 (typical to this site), total suspended particulate (TSP) concentration was in the range 15-40 mg m À3 (mean value 27.1 ± 8.3 mg m À3 ). Interestingly, aerosol BC had a mean concentration of 1.36 ± 0.99 mg m À3 and contributed $5.0 ± 1.3% to the composite aerosol mass. This large abundance of BC is found to have linkages to the human activities in the adjoining valley and to the boundary layer dynamics. Consequently, the inferred single scattering albedo lies in the range of 0.87 to 0.94 (mean value 0.90 ± 0.03), indicating significant aerosol absorption. The estimated aerosol radiative forcing was as low as À4.2 W m À2 at the surface, +0.7 W m À2 at the top of the atmosphere, implying an atmospheric forcing of +4.9 W m À2 . Though absolute value of the atmospheric forcing is quite small, which arises primarily from the very low AOD (or the column abundance of aerosols), the forcing efficiency (forcing per unit optical depth) was $88 W m À2 , which is attributed to the high BC mass fraction.