Telemedicine provides an attractive vision for tele-monitoring human health conditions and, thus, offers the opportunity for timely preventing chronic disease. A key limitation of promoting telemedicine in clinic application is the lack of a noninvasive med-tech and effective monitoring platform, which should be wearable and capable of high-performance tele-monitoring of health risk. Here we proposed a volatolomics-based telemedicine for continuously and noninvasively assessing human health status through continuously tracking the variation of volatile markers derived from human breath or skin. Particularly, a nanosensor-based flexible electronic was specifically designed to serve as a powerful platform for implementing the proposed cost-effective healthcare. An all-flexible and highly packed makeup (all functional units were integrated in a 2*2*0.19 cm3 plate) enables an electronic, compact configuration and the capability of resisting negative impact derived from customers’ daily movement. Notably, the nanosensor-based electronic demonstrates high specificity, quick response rate (t 90% = 4.5 s), and desirable low detection limit (down to 0.117 ppm) in continuous tele-monitoring chronic-disease-related volatile marker (e.g., acetone). Assisted by the power saved light fidelity (Li-Fi) communicating technology, a clinic proof on the specifically designed electronic for noninvasively and uninterrupted assessing potential health risk (e.g., diabetics) is successfully implemented, with the accuracy of around 81%. A further increase in the accuracy of prewarning is predicted by excluding the impact of individual differences such as the gender, age, and smoking status of the customer. These promising pilot results indicate a bright future for the tailor-made nanosensing-device-supported volatolomics-based telemedicine in preventing chronic diseases and increasing patients’ survival rate.
Yttria-stabilized zirconia (YSZ) based potentiometric gas sensors have been widely utilized for detecting NO x (NO and NO 2 ). Nevertheless, it is still remains challenging issue for YSZ-based sensors to sense total NO x due to the opposite response signals to NO and NO 2 . Herein, we report an efficient strategy to sense total NO x at high temperature (above 300 °C) by designing a dual functional sensing electrode (SE); namely, the SE will simultaneously convert NO (in NO x mixture) to NO 2 and electrocatalyze all of the obtained NO 2 to generate the response signal of total NO x . In comparison with those previously reported total NO x sensors, the proposed total NO x sensor will be featured with a simplified sensor configuration and desirable long-term stability. To confirm the practicability of the proposed strategy, the NO conversion rate of several metal oxides and their composites have been measured and it turns out that the Co 3 O 4 /NiO shows relatively high NO conversion rate. Further study indicates a YSZ-based sensor consisting of (Co 3 O 4 + 20 wt % NiO)-SE and Mn-based RE demonstrates satisfactory performance in detecting total NO x . For instance, analogous response magnitude to NO and NO 2 as well as the mixture of NO/NO 2 (within 35 ppm) is witnessed for the sensor; particularly, the sensor gives acceptable stability and response/recovery rate at the operating temperature of 500 °C within the examined period. In summary, the use of dual functional SE (e.g., Co 3 O 4 /NiO composite SE) indeed addressed those issues of concern in monitoring the level of total NO x and has provided a promising alternative way for designing future high-performance total NO x sensor.
Highlights A standalone-like smart device that can remotely track the variation of air pollutants in a power-saving way is created; Metal–organic framework-derived hollow polyhedral ZnO was successfully synthesized, allowing the created smart device to be highly selective and to sensitively track the variation of NO 2 concentration; A novel photoluminescence-enhanced Li-Fi telecommunication technique is proposed, offering the created smart device with the capability of long distance wireless communication. Abstract Remote tracking the variation of air quality in an effective way will be highly helpful to decrease the health risk of human short- and long-term exposures to air pollution. However, high power consumption and poor sensing performance remain the concerned issues, thereby limiting the scale-up in deploying air quality tracking networks. Herein, we report a standalone-like smart device that can remotely track the variation of air pollutants in a power-saving way. Brevity, the created smart device demonstrated satisfactory selectivity (against six kinds of representative exhaust gases or air pollutants), desirable response magnitude (164–100 ppm), and acceptable response/recovery rate (52.0/50.5 s), as well as linear response relationship to NO 2 . After aging for 2 weeks, the created device exhibited relatively stable sensing performance more than 3 months. Moreover, a photoluminescence-enhanced light fidelity (Li-Fi) telecommunication technique is proposed and the Li-Fi communication distance is significantly extended. Conclusively, our reported standalone-like smart device would sever as a powerful sensing platform to construct high-performance and low-power consumption air quality wireless sensor networks and to prevent air pollutant-induced diseases via a more effective and low-cost approach. Electronic supplementary material The online version of this article (10.1007/s40820-020-00551-w) contains supplementary material, which is available to authorized users.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.
hi@scite.ai
10624 S. Eastern Ave., Ste. A-614
Henderson, NV 89052, USA
Copyright © 2024 scite LLC. All rights reserved.
Made with 💙 for researchers
Part of the Research Solutions Family.