Topological semimetals host electronic structures with several band-contact points or lines and are generally expected to exhibit strong topological responses. Up to now, most work has been limited to non-magnetic materials and the interplay between topology and magnetism in this class of quantum materials has been largely unexplored. Here we utilize theoretical calculations, magnetotransport and angle-resolved photoemission spectroscopy to propose FeGeTe, a van der Waals material, as a candidate ferromagnetic (FM) nodal line semimetal. We find that the spin degree of freedom is fully quenched by the large FM polarization, but the line degeneracy is protected by crystalline symmetries that connect two orbitals in adjacent layers. This orbital-driven nodal line is tunable by spin orientation due to spin-orbit coupling and produces a large Berry curvature, which leads to a large anomalous Hall current, angle and factor. These results demonstrate that FM topological semimetals hold significant potential for spin- and orbital-dependent electronic functionalities.
In spintronics, two-dimensional van der Waals crystals constitute a most promising material class for long-distance spin transport or effective spin manipulation at room temperature. To realize all-vdW-material–based spintronic devices, however, vdW materials with itinerant ferromagnetism at room temperature are needed for spin current generation and thereby serve as an effective spin source. We report theoretical design and experimental realization of a iron-based vdW material, Fe4GeTe2, showing a nearly room temperature ferromagnetic order, together with a large magnetization and high conductivity. These properties are well retained even in cleaved crystals down to seven layers, with notable improvement in perpendicular magnetic anisotropy. Our findings highlight Fe4GeTe2 and its nanometer-thick crystals as a promising candidate for spin source operation at nearly room temperature and hold promise to further increase Tc in vdW ferromagnets by theory-guided material discovery.
We present a fully automatic framework that digitizes a complete 3D head with hair from a single unconstrained image. Our system offers a practical and consumer-friendly end-to-end solution for avatar personalization in gaming and social VR applications. The reconstructed models include secondary components (eyes, teeth, tongue, and gums) and provide animation-friendly blendshapes and joint-based rigs. While the generated face is a high-quality textured mesh, we propose a versatile and efficient polygonal strips (polystrips) representation for the hair. Polystrips are suitable for an extremely wide range of hairstyles and textures and are compatible with existing game engines for real-time rendering. In addition to integrating state-of-the-art advances in facial shape modeling and appearance inference, we propose a novel single-view hair generation pipeline, based on 3D-model and texture retrieval, shape refinement, and polystrip patching optimization. The performance of our hairstyle retrieval is enhanced using a deep convolutional neural network for semantic hair attribute classification. Our generated models are visually comparable to state-of-the-art game characters designed by professional artists. For real-time settings, we demonstrate the flexibility of polystrips in handling hairstyle variations, as opposed to conventional strand-based representations. We further show the effectiveness of our approach on a large number of images taken in the wild, and how compelling avatars can be easily created by anyone.
Essential resources of many rare metals including copper, zinc, molybdenum, silver and gold occur in natural sulfide mineral deposits. Understanding the origin of these metal resources has been limited by a lack of data about the geochemistry of sulfur, the most important and abundant element of ore deposits. We report the first directly measured sulfur concentrations in high-temperature fluids, together with their ore-metal contents, using a new method for sulfur quantification in fluid inclusions by laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS). Co-genetic brine and vapor inclusions from magmatic-hydrothermal ore deposits and granitic intrusions show an excess of sulfur over ore metals, as required for efficient oremineral precipitation. The results demonstrate that S, Cu and Au are highly enriched in vapor-like magmatic fluids, implying that such low-salinity fluids are the key agent for the formation of porphyry copper and epithermal gold deposits.
The accuracy and precision of micro-analysis of sulfur (S), chlorine (Cl) and bromine (Br) in quartz-hosted fluid inclusions by laser ablation (LA) inductively coupled plasma mass spectrometry (ICP-MS) was tested. A scapolite mineral sample (Sca17) can be used as standard reference material (SRM) for the determination of Cl and Br, and NIST610 glass for S determination in fluid inclusions. We found that laser ablation of quartz and UV irradiation in the ablation cell produced elevated background signals of S and to a lesser amount of Cl and Br due to remobilization of these elements from the inside surfaces of the ablation Page 2 chamber. Careful cleaning of the ablation chamber with nitric acid and by UV irradiation results in a 10 times lower S contamination signal and improves fluid inclusion analysis by reducing the detection limit for S by 50%. Micro-analysis of liquid and vapor inclusions synthesized in two different laboratories produce good accuracies of S, Cl, and Br. Analytical uncertainties based on numerous analyses of individual synthetic fluid inclusions in one assemblage are 17-44 % (RSD) for the sulfur concentration, and 6-26 % for Br/Cl ratios. Limits of detection (LOD) in 30 μm diameter liquid inclusions with densities of 0.99-1.02 g/cm 3 are in the range of 60 μg/g for S, 250 μg/g for Cl, and 15 μg/g for Br. LOD's in similar sized vapor inclusions with a density of 0.33 g/cm 3 are at least an order of magnitude poorer. Based on the investigated natural brine inclusion assemblages, the precisions of Br/Cl ratios (4-9 % RSD) is adequate to determine the source of salinity in different ore-forming fluids.
The quantification capabilities for sulfur microanalysis in quartz-hosted fluid inclusions were investigated with laser ablation (LA) inductively coupled plasma quadrupole mass spectrometry (ICP-Q-MS) and ICP sector field mass spectrometry (ICP-SF-MS) allowing resolution of sulfur from polyatomic interferences. A scapolite mineral sample was used to determine the sulfur concentration in NIST SRM 610 (570 AE 70 mg g À1 ), which was further validated using EPMA and then used as standard reference material for the fluid inclusion analysis. The sulfur concentration in an assemblage of brine inclusions from a quartz-molybdenum vein was determined to be 5900 AE 2000 mg g À1 measuring 17 inclusions with the ICP-SF-MS and 13 inclusions with the ICP-Q-MS instrument. The agreement between the two ICP-MS instruments for sulfur was $5% and well within the overall precision of 35% relative standard deviation. The precision and accuracy was not limited by interferences, but by a so far unknown sulfur contamination source when ablating the host mineral quartz. Due to this contamination, a careful baseline correction is necessary which is described and discussed in detail. Nevertheless, the method developed to determine sulfur maintains the multi-element capabilities for individual fluid inclusions. Limits of detection for sulfur are correlated with the inclusion mass and were found to be $ 30-100 mg g À1 for 60 mm inclusions.
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