Radiometric ages for undated parts of the volcanic succession and intrusions in West Greenland were obtained by the 40Ar–39Ar incremental heating method. Acceptable crystallization ages were obtained for 27 samples. Combined with published results the new data provide a volcanic stratigraphy correlatable throughout the Nuussuaq Basin. The thick onshore volcanic pile consists of four widespread formations: 62.5–61 Ma picrites (Vaigat Formation), 61–60 Ma depleted basalts (Maligât Formation and the Hellefisk-1 well), 60–58 Ma less-depleted basalts (Svartenhuk Formation) and 56–54 Ma enriched basalts (Naqerloq Formation). Two local successions comprise 53.5 Ma alkali basalts (Erqua Formation) and 38.7 Ma transitional basalts (Talerua Member). A central volcano developed on Ubekendt Ejland, leading to the Sarqâta qáqâ gabbro-granophyre intrusion at 57–55 Ma. Pre-break-up volcanism took place further south as early as 64–63 Ma. The offshore volcanic succession most probably comprises the known onshore succession plus some younger lavas. The change in spreading direction near the Paleocene–Eocene boundary took place west of the Nuussuaq Basin c. 56.2 Ma. Some tectonomagmatic events are correlatable across the entire North Atlantic Igneous Province. A quiescent 58–56 Ma period correlates with similar periods in East Greenland and the Faroes, and the Naqerloq Formation is coeval with the Eocene basalts in East Greenland. The Paleocene and Eocene tholeiitic basalts are distinguishable chemically; in early Eocene time, mantle typical of the Iceland plume seems to have extended beneath the whole West Greenland margin as well as the central East Greenland margin.

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The West Greenland/Baffin Island Tertiary volcanic province differs from other CFB provinces in containing an unusually high proportion (30-50% by volume) of magnesian picritic lavas and hyaloclastites. Olivine-liquid equilibrium considerations suggest the presence during the earlier stages of eruption of picritic melts with MgO contents as high as 20%. Calculations based on McKenzie-Bickle melting models point to high degrees of melting (24-30%) at depths of 60-90 km in the underlying mantle, and require potential temp-" eratures of 1540-1600°C. Such high potential temperatures are inconsistent with reconstructions that attribute the West Greenland volcanism to melting on the margins of the incipient Iceland plume-head. The distribution of Tertiary volcanic activity in Greenland, in particular its relation to Mesozoic-Tertiary extensional basins, indicates that lithospheric structure plays a part in determining where the plume-head can undergo melting. But to explain the restriction of high-temperature picrites to West Greenland, together with their distinctive trace element geochemistry, it is necessary to invoke (a) either an elongated Icelandic plume initially extending as far as West Greenland or a short-lived precursory plume head that developed directly beneath West Greenland, and (b) an active extensional regime that allowed rapid access of picritic melts to the surface.

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