Microrods of the ferrosulfide minerals greigite (Fe3S4) and marcasite (FeS2) are selectively synthesized by an in situ magnetic‐field‐assisted hydrothermal route. Each complex microrod is composed of fine building blocks with different shapes. The unique magnetic properties of the microrods and electrical performance of a single microrod are studied. The results demonstrate that the magnetic properties of the ferrosulfide minerals are strongly related to their corresponding microstructures. The value of the low‐temperature transition increases as the greigite component in the product decreases. The combination of small‐molecule sulfur precursors and an applied magnetic field makes possible the selective synthesis of ferrosulfide minerals with different phases and distinct microstructures, underlining the fact that the magnetic field can be a useful tool as well as an independent parameter for the phase‐selective synthesis and self‐assembly of inorganic building blocks in solution chemistry.
High-sensitive measurement of radio-frequency (RF) electric field is available via the electromagnetically induced transparency (EIT) effect of Rydberg atom at room-temperature, which has been developed to be a promising atomic RF receiver. In this Letter, we investigate the credibility of the digital communication via this quantum-based antenna over the entire continuously tunable RF-carrier. Our experiment shows that digital communication at a rate of 500 kbps performs reliably within a tunable bandwidth of 200 MHz at carrier 10.22 GHz and a bit error rate (BER) appears out of this range, for example, the BER runs up to 15% at RF-detuning ±150 MHz. In the measurement, the time-variant RF field is retrieved by detecting the density of the probe laser at the center frequency of RF-induced symmetric or asymmetric Autler-Townes splitting in EIT. Prior to the digital test, we have studied the RF-receiving quality versus the physical ambiance and found that a choice of linear gain response to the RF-amplitude can suppress the signal distortion and the modulating signal is able to be decoded as fast as up to 500 kHz in the tunable bandwidth. Our checkout consolidates the physical foundation for a reliable communication and spectrum sensing over the broadband RFE-field signal in free-space can be captured by measuring the transmission of a probe laser in a condition of a Rydberg EIT. Owing to unique advantages of free-space RF field sensing, the quantum receiver has great significance compared with conventional electronics-based receivers, including but not limited to the weak signal, long-distance communication in free space or via a fiber link. All the principle experiments of communication were performed over carrier of an optimized resonant frequency of Rydberg states [11][12][13].
We studied the effect of particle size on the structure and magnetic properties of La0.6Pb0.4MnO3 compounds with particle diameters varying from 5to100nm. With decreasing particle size, the increase of the rhombohedral distortion narrows the bandwidth WO2p and hence results in the decrease of ferromagnetic transition temperature. At the same time, the magnetic domain structure evolves from multidomain to single domain, and finally a superparamagnetic behavior is detected. The critical single domain size determined by experiment is about 25nm, and the critical superparamagnetic behavior size obtained by calculation is 5.8nm. It is found that the variation of coercivity is related to the evolution of magnetic domain states with particle size, and the saturation magnetization decreases significantly due to the increasing contribution of the surface effect with decreasing particle size.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.