Self-oscillation capable of maintaining periodic motion upon constant stimulus has potential applications in the fields of autonomous robotics, energy-generation devices, mechano-logistic devices, sensors, and so on. Inspired by the active jumping of kangaroos and frogs in nature, we proposed a self-jumping liquid crystal elastomer (LCE) balloon under steady illumination. Based on the balloon contact model and dynamic LCE model, a nonlinear dynamic model of a self-jumping LCE balloon under steady illumination was formulated and numerically calculated by the Runge–Kutta method. The results indicated that there exist two typical motion regimes for LCE balloon under steady illumination: the static regime and the self-jumping regime. The self-jumping of LCE balloon originates from its expansion during contact with a rigid surface, and the self-jumping can be maintained by absorbing light energy to compensate for the damping dissipation. In addition, the critical conditions for triggering self-jumping and the effects of several key system parameters on its frequency and amplitude were investigated in detail. The self-jumping LCE hollow balloon with larger internal space has greater potential to carry goods or equipment, and may open a new insight into the development of mobile robotics, soft robotics, sensors, controlled drug delivery, and other miniature device applications.
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