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Three‐dimensional modeling of the gas–solid flow in a spout‐fluid bed is conducted at the particle‐scale level. Both the local and systematic dispersion behaviors of solid phase are initially investigated. Then, the solid circulating and resident behaviors are discussed. The results demonstrate that vigorously lateral solid dispersion appears in the spout region and the periphery of the fountain, whereas intensely vertical dispersion exists in the central region of the bed. Moreover, the inlet configuration of bed strongly affects the distribution of lateral dispersion, while its influence on the vertical one disappears in the fountain. Strong anisotropy of solid dispersion along the three directions is obtained. Systematic dispersion intensity along the vertical direction is an order of magnitude larger than the lateral one. In addition, two circulating patterns of solid phase can be identified. Solid residence time is the smallest in the spout region and the largest in the bottom corner. © 2014 American Institute of Chemical Engineers AIChE J, 60: 2788–2804, 2014

A compressible direct numerical simulation (DNS) solver for pulverized coal combustion has been developed and used to study a pulverized coal jet flame with a Reynolds number of 28 284 based on the nozzle diameter. An eighth-order center differential scheme combined with an explicit tenth-order filter is used for spatial discretization. The classical fourth-order Runge−Kutta method is used for time integration. The characteristic non-reflecting boundary conditions are used to describe the boundary conditions. A comprehensive model for coal combustion is applied, and the reaction mechanism of CH 4 with five species and two-step reactions is adopted for gas-phase combustion. The grid system has been carefully designed to make sure that turbulent scales and chemical reaction scales are reasonably resolved and the point-source assumptions of particles are valid. The simulation is partially validated against the experiment, and the particle behavior is investigated. It is found that, in the upstream region, the reaction rate is quite scattered and a single particle is found inside the burning flame to form an individual particle combustion mode. While in the downstream region, the reaction zone is more continuous, with a large number of particles enclosed, which characterizes the group combustion mode. Conditional statistics with respect to the mixture fraction are also obtained to provide insights into coal combustion and the related models.

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Abstract. The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) was used to study the effect of extreme weather events on ozone in the US for historical (2001–2010) and future (2046–2055) periods under the RCP8.5 scenario. During extreme weather events, including heat waves, atmospheric stagnation, and their compound events, ozone concentration is much higher compared to the non-extreme events period. A striking enhancement of effect during compound events is revealed when heat wave and stagnation occur simultaneously as both high temperature and low wind speed promote the production of high ozone concentrations. In regions with high emissions, compound extreme events can shift the high-end tails of the probability density functions (PDFs) of ozone to even higher values to generate extreme ozone episodes. In regions with low emissions, extreme events can still increase high-ozone frequency but the high-end tails of the PDFs are constrained by the low emissions. Despite the large anthropogenic emission reduction projected for the future, compound events increase ozone more than the single events by 10 to 13 %, comparable to the present, and high-ozone episodes with a maximum daily 8 h average (MDA8) ozone concentration over 70 ppbv are not eliminated. Using the CMIP5 multi-model ensemble, the frequency of compound events is found to increase more dominantly compared to the increased frequency of single events in the future over the US, Europe, and China. High-ozone episodes will likely continue in the future due to increases in both frequency and intensity of extreme events, despite reductions in anthropogenic emissions of its precursors. However, the latter could reduce or eliminate extreme ozone episodes; thus improving projections of compound events and their impacts on extreme ozone may better constrain future projections of extreme ozone episodes that have detrimental effects on human health.