Non-volatile, bidirectional, all-optical switching in a phase-change metamaterial delivers high-contrast transmission and reflection modulation at near- to mid-infrared wavelengths in device structures down to ≈1/27 of a wavelength thick.
According to Huygens' superposition principle, light beams traveling in a linear medium will pass though one another without mutual disturbance. Indeed, it is widely held that controlling light signals with light requires intense laser fields to facilitate beam interactions in nonlinear media, where the superposition principle can be broken. We demonstrate here that two coherent beams of light of arbitrarily low intensity can interact on a metamaterial layer of nanoscale thickness in such a way that one beam modulates the intensity of the other. We show that the interference of beams can eliminate the plasmonic Joule losses of light energy in the metamaterial or, in contrast, can lead to almost total absorbtion of light. Applications of this phenomenon may lie in ultrafast all-optical pulse-recovery devices, coherence filters and THz-bandwidth light-by-light modulators
Current efforts in metamaterials research focus on attaining dynamic functionalities such as tunability, switching and modulation of electromagnetic waves. To this end, various approaches have emerged, including embedded varactors, phase-change media, the use of liquid crystals, electrical modulation with graphene and superconductors, and carrier injection or depletion in semiconductor substrates. However, tuning, switching and modulating metamaterial properties in the visible and near-infrared range remain major technological challenges: indeed, the existing microelectromechanical solutions used for the sub-terahertz and terahertz regimes cannot be shrunk by two to three orders of magnitude to enter the optical spectral range. Here, we develop a new type of metamaterial operating in the optical part of the spectrum that is three orders of magnitude faster than previously reported electrically reconfigurable metamaterials. The metamaterial is actuated by electrostatic forces arising from the application of only a few volts to its nanoscale building blocks-the plasmonic metamolecules-that are supported by pairs of parallel strings cut from a flexible silicon nitride membrane of nanoscale thickness. These strings, of picogram mass, can be driven synchronously to megahertz frequencies to electromechanically reconfigure the metamolecules and dramatically change the transmission and reflection spectra of the metamaterial. The metamaterial's colossal electro-optical response (on the order of 10(-5)-10(-6) m V(-1)) allows for either fast continuous tuning of its optical properties (up to 8% optical signal modulation at up to megahertz rates) or high-contrast irreversible switching in a device only 100 nm thick, without the need for external polarizers and analysers.
Environmental light is the 'zeitgeber' (time-giver) of circadian behaviour. Constant darkness is considered a 'free-running' circadian state. Mammals encounter constant darkness during hibernation. Ablation of the master clock synchronizer, the suprachiasmatic nucleus, abolishes torpor, a hibernation-like state, implicating the circadian clock in this phenomenon. Here we report a mechanism by which constant darkness regulates the gene expression of fat catabolic enzymes in mice. Genes for murine procolipase (mClps) and pancreatic lipase-related protein 2 (mPlrp2) are activated in a circadian manner in peripheral organs during 12 h dark:12 h dark (DD) but not light-dark (LD) cycles. This mechanism is deregulated in circadian-deficient mPer1-/-/mPer2m/m mice. We identified circadian-regulated 5'-AMP, which is elevated in the blood of DD mice, as a key mediator of this response. Synthetic 5'-AMP induced torpor and mClps expression in LD animals. Torpor induced by metabolic stress was associated with elevated 5'-AMP levels in DD mice. Levels of glucose and non-esterified fatty acid in the blood are reversed in DD and LD mice. Induction of mClps expression by 5'-AMP in LD mice was reciprocally linked to blood glucose levels. Our findings uncover a circadian metabolic rhythm in mammals.
We study the angular scattering properties of individual core-shell nanoparticles that support simultaneously both electric and optically-induced magnetic resonances of different orders. In contrast to the approach to suppress the backward scattering and enhance the forward scattering relying on overlapping electric and magnetic dipoles, we reveal that the directionality of the forward scattering can be further improved through the interferences of higher order electric and magnetic modes. Since the major contributing electric and magnetic responses can be tuned to close magnitudes, ultra-directional forward scattering can be achieved by single nanoparticles without compromising the feature of backward scattering suppression, which may offer new opportunities for nanoantennas, photovoltaic devices, bio-sensing and many other interdisciplinary researches.
Metamaterials, as artificially structured materials composed of subwavelength arrays of resonant unit cells, can exhibit exotic properties beyond those accessible to natural materials. They were initially proposed for challenging fundamental laws and demonstrating negative refraction in the microwave regime, and subsequently exploited as a versatile platform to manipulate electromagnetic waves throughout the spectrum via their extreme scalability. Over the past decade, research into metamaterials has been extended to a search for real-world applications, leading to the concept of metadevices, defined as metamaterial-based devices that can operate in an active manner. Due to their subwavelength scale, metamaterials present intriguing strategies for active tuning and provide flat, high-efficiency alternatives to conventional optical systems based on bulky components. In this topical review, we summarize the development of active metamaterials and metadevices ranging from microwave to visible wavelengths, including milestones as well as the state of the art. We survey tuning strategies based on mechanical reconfiguration and incorporation with active materials such as varactor diodes, semiconductors, liquid crystals, phase change materials, superconductors, and two-dimensional materials under various external stimuli, and discuss their fascinating advantages and potential challenges to be confronted. Finally, future prospects together with several emerging tuning strategies and materials are presented at the end.
Periodic nanostructuring can enhance the optical nonlinearity of plasmonic metals by several orders of magnitude. By patterning a gold film, the largest sub-100 femtosecond nonlinearity is achieved, which is suitable for terahertz rate all-optical data processing as well as ultrafast optical limiters and saturable absorbers.
Optical responses in conventional metamaterials based on plasmonic metal nanostructures are inevitably accompanied by Joule losses, which obstruct practical applications by limiting resonance quality factors and compromising the efficiency of metamaterial devices. Here we experimentally demonstrate a fully-dielectric metamaterial that exhibits a 'trapped mode' resonance at optical frequencies, founded upon the excitation by incident light of anti-parallel displacement currents in metamolecules comprising pairs of parallel, geometrically dissimilar dielectric nano-bars. The phenomenon is demonstrated in the near-infrared part of the spectrum using silicon, showing that in principle strong, lossless resonant responses are possible anywhere in the optical spectral range.
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