The exploration of flexible and lightweight electromagnetic interference (EMI) shielding materials with excellent shielding effectiveness, as a means to effectively alleviate electromagnetic pollution, is still a tremendous challenge. This paper proposes a conducting material named the textured Ni-encapsulated carbon tube, which can be applied in EMI shielding material by being inserted in the center of a poly(dimethysiloxane) (PDMS) polymer. We demonstrated that Pd 2+ could be absorbed by the active groups on the plant fiber surface to catalyze the reduction of Ni 2+ as a catalytic center by means of a textured Ni-encapsulated plant fiber. Owing to the outstanding heat-conducting capability of the Ni coating, the inner plant fiber was carbonized and attached to the Ni-tube inside the surface during annealing. To be precise, the textured Ni-encapsulated C tube was fabricated successfully after annealing at 300 °C. On further increasing the annealing temperature, the C tube disappeared gradually with the Ni coating being oxidized to NiO. Of note, the C tube acted as a support layer for the external Ni coating, providing sufficient mechanical strength. When combined with the coating PDMS layer, a flexible and lightweight EMI shielding material is fabricated successfully. It displays an outstanding EMI shielding effectiveness of 31.34 dB and a higher specific shielding efficiency of 27.5 dB•cm 3 /g, especially showing excellent mechanical property and flexibility with only 2 mm thickness. This study provides a new method to fabricate outstanding EMI shielding materials.
A triboelectric nanogenerator (TENG) collects thriftless mechanical energy from the surrounding environment and transforms it into electrical energy. This work demonstrated a feasible method for metallizing the polylactic acid (PLA) surface, which was subsequently used as a biomaterial-based TENG electrode material. We demonstrated that microcellular holes and hydrophilic groups (−C-OH and −COOH) were introduced on an alkali-treated PLA sheet surface, subsequently used to absorb Pd 2+ by means of covalent bonds, which could serve as catalytic centers for the reduction of Ni 2+ . Of note, the Ni-layer deposition mechanism represents a typical island-like growth pattern. To be precise, a Ni-coated PLA sheet was fabricated successfully and used as a TENG electrode material. The device had excellent performances, with a maximum output voltage of about 5.1 V, obtained from 6% strain (the corresponding stress is 32.4 kPa) on the PDMS layer. Furthermore, it revealed that under a stress of 0.14−32.4 kPa and strain of 1.3−6%, a linear regression relation existed between the output voltage and the dielectric material strain, and it was found that the density of electrostatic charge formed on the TENG material surface is 4.1 × 10 6 C/m 2 . Additionally, the as-fabricated TENG equipment was attached to various positions of the human body and lab to demonstrate the electrical energy obtained from the mechanical movement. It was also used for real-time demonstrations as a self-powered body-tracking device application which may be beneficial in tracking human position counters during self-powered and emergency exercise movements.
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