We report about the existence of magneto-acoustic pulses propagating in a 200-nm-thick ferromagnetic nickel film excited with 120 fs laser pulses. They result from the coupling between the magnetization of the ferromagnetic film and the longitudinal acoustic waves associated to the propagation of the lattice deformation induced by the femtosecond laser pulses. The magneto-acoustic pulses are detected from both the front and back sides of the film, using the time-resolved magnetooptical Kerr technique, measuring both the time dependent rotation and ellipticity. We show that the propagating acoustic pulse couples efficiently to the magnetization and is strong enough to induce a precession of the magnetization. It is due to a transient change of the crystalline anisotropy associated to the lattice deformation. It is shown that the results can be interpreted by combining the concepts of acoustic pulse propagation and ultrafast magnetization dynamics.The technology of information and communication constantly needs to improve the speed and density of memory devices. Towards that goal, intense researches are being carried out for manipulating the spins in magnetic materials using various excitation methods like the use of external magnetic field pulses [1][2][3]. Alternatively, femtosecond laser pulses have been utilized to induce an ultrafast demagnetization via a sudden and abrupt change of the temperature of the magnetic material [4-10], or using the inverse Faraday effect [11,12]. This new field of magnetism, named "femtomagnetism" [13,14], uses photons to directly manipulate magnetic structures with a temporal resolution of a few femtosecond. The demagnetization can then be used to modify the anisotropy of the magnetic material [15] which leads to a reorientation of the magnetization vector followed by its precession and damping in the direction opposite to the initial one [10,16,17]. In spite of their versatility, due to the various laser wavelengths and pulse durations, magnetooptical methods are limited by the absorption depth of photons. For application purposes, it is a disadvantage for controlling devices at long distances, particularly in opaque materials like ferromagnetic metals.In the present work we explore an alternative way of controlling the magnetization, based on magnetoacoustic performed at room temperature in ferromagnetic films. It is known that strain pulses, corresponding to a lattice deformation of a material, can be generated with a laser pulse, a subject which has been extensively studied theoretically and experimentally [18][19][20], since the pioneering works of Thomsen et al. [21,22]. The relative amplitude of these strain pulses can be as large as 10 −3 . Such acoustic waves have been used for perturbing the magnetic properties of a dilute magnetic semiconductor material, at low temperature and with a very low efficiency [23]. Here we show that one can efficiently use the strain pulses that propagates over long distances in ferromagnetic metals at room temperature and induce very large ...

Controlling the angular momentum of spins with very short external perturbations is a key issue in modern magnetism. For example it allows manipulating the magnetization for recording purposes or for inducing high frequency spin torque oscillations. Towards that purpose it is essential to modify and control the angular momentum of the magnetization which precesses around the resultant effective magnetic field. That can be achieved with very short external magnetic field pulses or using intrinsically coupled magnetic structures, resulting in a transfer of spin torque. Here we show that using picosecond acoustic pulses is a versatile and efficient way of controlling the spin angular momentum in ferromagnets. Two or three acoustic pulses, generated by femtosecond laser pulses, allow suppressing or enhancing the magnetic precession at any arbitrary time by precisely controlling the delays and amplitudes of the optical pulses. A formal analogy with a two dimensional pendulum allows us explaining the complex trajectory of the magnetic vector perturbed by the acoustic pulses.

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An ultrafast spin demagnetization process of an amorphous Tb35Fe65 alloy film has been investigated by means of an all-optical pump-probe technique. Interestingly, steplike demagnetization on a subpicosecond time scale is observed before a much slower change on a time scale of tens of picoseconds. The steplike demagnetization at the subpicosecond scale is explained by the extended three-temperature model considering the interaction between a nonthermal electron and a spin system. The characteristic of subpicosecond demagnetization of TbFe alloy film is expected to be very useful in the manipulation of the spin state in ultrafast regime.

We have investigated the ultrafast magnetization dynamics of L10-ordered Fe50Pt50 thin film by means of a time-resolved magneto-optical Kerr effect measurement. We have found a high Gilbert damping value of α∼0.26, together with a very high precession frequency of f∼85 GHz and the shortest relaxation characteristic time of τ∼6.5 ps ever reported. We believe that L10-ordered FePt film with the unique property of a very high precession frequency and the shortest relaxation time will be very useful for the realization of picosecond spin switching.

The magnetization dynamics of perpendicularly magnetized FePt films is studied using both magnetic-field-induction and all-optical methods. A critically damped trajectory was observed in this system, where the precession ended within subnanoseconds after a single large oscillation. Using the Landau–Lifshitz–Gilbert (LLG) calculation with an experimental configuration, the effective anisotropy and damping constant were obtained. A damping constant of approximately 0.2 was determined after both a magnetic field and a laser pulse were used. The laser-induced real-space trajectory was well explained by the modified LLG calculation taking into account the demagnetization and time-dependent anisotropy.

We report the anharmonic angstrom dynamics of self-assembled Au nanoparticles (Au:NPs) away from a nickel surface on top of which they are coupled by their near-field interaction. The deformation and the oscillatory excursion away from the surface are induced by picosecond acoustic pulses and probed at the surface plasmon resonance with femtosecond laser pulses. The overall dynamics are due to an efficient transfer of translational momentum from the Ni surface to the Au:NPs, therefore avoiding usual thermal effects and energy redistribution among the electronic states. Two modes are clearly revealed by the oscillatory shift of the Au:NPs surface plasmon resonance-the quadrupole deformation mode due to the transient ellipsoid shape and the excursion mode when the Au:NPs bounce away from the surface. We find that, contrary to the quadrupole mode, the excursion mode is sensitive to the distance between Au:NPs and Ni. Importantly, the excursion dynamics display a nonsinusoidal motion that cannot be explained by a standard harmonic potential model. A detailed modeling of the dynamics using a Hamaker-type Lennard-Jones potential between two media is performed, showing that each Au:NPs coherently evolves in a nearly one-dimensional anharmonic potential with a total excursion of ∼1 Å. This excursion induces a shift of the surface plasmon resonance detectable because of the strong near-field interaction. This general method of observing the spatiotemporal dynamics with angstrom and picosecond resolutions can be directly transposed to many nanostructures or biosystems to reveal the interaction and contact mechanism with their surrounding medium while remaining in their fundamental electronic states.

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