Optical parametric oscillation is a nonlinear process that enables coherent generation of 'signal' and 'idler' waves, shifted in frequency from the pump wave. Efficient parametric conversion is the paradigm for the generation of twin or entangled photons for quantum optics applications such as quantum cryptography, or for the generation of new frequencies in spectral domains not accessible by existing devices. Rapid development in the field of quantum information requires monolithic, alignment-free sources that enable efficient coupling into optical fibres and possibly electrical injection. During the past decade, much effort has been devoted to the development of integrated devices for quantum information and to the realization of all-semiconductor parametric oscillators. Nevertheless, at present optical parametric oscillators typically rely on nonlinear crystals placed into complex external cavities, and pumped by powerful external lasers. Long interaction lengths are typically required and the phase mismatch between the parametric waves propagating at different velocities results in poor parametric conversion efficiencies. Here we report the demonstration of parametric oscillation in a monolithic semiconductor triple microcavity with signal, pump and idler waves propagating along the vertical direction of the nanostructure. Alternatively, signal and idler beams can also be collected at finite angles, allowing the generation of entangled photon pairs. The pump threshold intensity is low enough to envisage the realization of an all-semiconductor electrically pumped micro-parametric oscillator.
We present an experimental and theoretical study of the existence of acoustic phonon sidebands in the emission line of single self-assembled InAs/GaAs quantum dots. Temperature-dependent photoluminescence measurements reveal a deviation from a Lorentzian profile with the appearance of lateral sidebands. We obtain an excellent agreement with calculations done in the framework of the Huang-Rhys formalism. We conclude that the only relevant parameter for the observation of acoustic phonon sidebands is the linewidth of the central zero-phonon line. At high temperature, the quasi-Lorentzian quantum dot line appears to be fully determined by the acoustic phonon sidebands
The amplification of spontaneous emission is used to initiate laser action. As the phase of spontaneous emission is random, the phase of the coherent laser emission (the carrier phase) will also be random each time laser action begins. This prevents phase-resolved detection of the laser field. Here, we demonstrate how the carrier phase can be fixed in a semiconductor laser: a quantum cascade laser (QCL). This is performed by injection seeding a QCL with coherent terahertz pulses, which forces laser action to start on a fixed phase. This permits the emitted laser field to be synchronously sampled with a femtosecond laser beam, and measured in the time domain. We observe the phase-resolved buildup of the laser field, which can give insights into the laser dynamics. In addition, as the electric field oscillations are directly measured in the time domain, QCLs can now be used as sources for time-domain spectroscopy.
Nonlinear couplings between photons and electrons in new materials give rise to a wealth of interesting nonlinear phenomena [1]. This includes frequency mixing, optical rectification or nonlinear current generation, which are of particular interest for generating radiation in spectral regions that are difficult to access, such as the terahertz gap. Owing to its specific linear dispersion and high electron mobility at room temperature, graphene is particularly attractive for realizing strong nonlinear effects [2]. However, since graphene is a centrosymmetric material, second-order nonlinearities a priori cancel, which imposes to rely on less attractive third-order nonlinearities [3]. It was nevertheless recently demonstrated that dc-second-order nonlinear currents [4] as well as ultrafast ac-currents [5] can be generated in graphene under optical excitation. The asymmetry is introduced by the excitation at oblique incidence, resulting in the transfer of photon momentum to the electron system, known as the
The generation of ultrashort pulses from quantum cascade lasers (QCLs) has proved to be challenging. It has been suggested that the ultrafast electron dynamics of these devices is the limiting factor for modelocking and hence pulse formation. Even so, clear modelocking of terahertz (THz) QCLs has been recently demonstrated but the exact mechanism for pulse generation is not fully understood. Here we demonstrate that the dominant factor necessary for active pulse generation is in fact the synchronization between the propagating electronic modulation and the generated THz pulse in the QCL. By using phase resolved detection of the electric field in QCLs embedded in metal-metal waveguides, we demonstrate that active modelocking requires the phase velocity of the microwave round trip modulation to equal the group velocity of the THz pulse. This allows the THz pulse to propagate in phase with the microwave modulation along the gain medium, permitting short pulse generation. Modelocking was performed on QCLs employing phonon depopulation active regions, permitting coherent detection of large gain bandwidths (500 GHz), and the generation of 11 ps pulses centered around 2.6 THz when the above 'phase-matching' condition is satisfied. This work brings an enhanced understanding of QCL modelocking and will permit new concepts to be explored to generate shorter and more intense pulses from mid-infrared, as well as THz, QCLs.
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