Electron-phonon interaction is a major source of optical dephasing in semiconductor quantum dots. Within a density matrix theory the electron-phonon interaction is considered up to the second order of a correlation expansion, allowing the calculation of the quantum kinetic dephasing dynamics of optically induced nonlinearities in GaAs quantum dots for arbitrary pulse strengths and shapes. We find Rabi oscillations renormalized and a damping that depends on the input pulse strength, a behavior not known from exponential dephasing mechanisms.

Plasmon modes of the exact same individual gold nanoprisms are investigated through combined nanometer-resolved electron energy-loss spectroscopy (EELS) and cathodoluminescence (CL) measurements. We show that CL only probes the radiative modes, in contrast to EELS, which additionally reveals dark modes. The combination of both techniques on the same particles thus provides complementary information and also demonstrates that although the radiative modes give rise to very similar spatial distributions when probed by EELS or CL, their resonant energies appear to be different. We trace this phenomenon back to plasmon dissipation, which affects in different ways the plasmon signatures probed by these techniques. Our experiments are in agreement with electromagnetic numerical simulations and can be further interpreted within the framework of a quasistatic analytical model. We therefore demonstrate that CL and EELS are closely related to optical scattering and extinction, respectively, with the addition of nanometer spatial resolution.

Optical experiments on second-harmonic generation from split-ring-resonator square arrays show a nonmonotonic dependence of the conversion efficiency on the lattice constant. This finding is interpreted in terms of a competition between dilution effects and linewidth or near-field changes due to interactions among the individual elements in the array.

Plasmonic nanoantennas provide unprecedented opportunities to concentrate light fields in subwavelength-sized volumes. By placing a nonlinear dielectric nanoparticle in such a hot spot, one can hope to take advantage of both the field enhancement provided by nanoantennas and the large, nonlinear optical susceptibility of dielectric nanoparticles. To test this concept, we combine gold gap nanoantennas with second-order, nonlinear zinc sulfide nanoparticles, and perform second harmonic generation (SHG) spectroscopy on the combined hybrid dielectric/plasmonic nanoantennas as well as on the individual constituents. We find that SHG from the bare gold nanoantennas, even though it should be forbidden due to symmetry reasons, is several orders of magnitude larger than that of the bare zinc sulfide nanoparticles. Even stronger second harmonic signals are generated by the hybrid dielectric/plasmonic nanoantennas. Control experiments with nanoantennas containing linear lanthanum fluoride nanoparticles reveal; however, that the increased SHG efficiency of the hybrid dielectric/plasmonic nanoantennas does not depend on the nonlinear optical susceptibility of the dielectric nanoparticles but is an effect of the modification of the dielectric environment. The combination of a hybrid dielectric/plasmonic nanoantenna, which is only resonant for the incoming pump light field, with a second nanoantenna, which is resonant for the generated second harmonic light, allows for a further increase in the efficiency of SHG. As the second nanoantenna mediates the coupling of the second harmonic light to the far field, this double-resonant approach also provides us with control over the polarization of the generated light.

We study the quantum properties and statistics of photons emitted by a quantum-dot biexciton inside a cavity. In the biexciton-exciton cascade, fine-structure splitting between exciton levels degrades polarization-entanglement for the emitted pair of photons. However, here we show that the polarization-entanglement can be preserved in such a system through simultaneous emission of two degenerate photons into cavity modes tuned to half the biexciton energy. Based on detailed theoretical calculations for realistic quantum-dot and cavity parameters, we quantify the degree of achievable entanglement.

We present a microscopic many-particle theory for the dephasing of coherent intersubband excitations in semiconductor quantum wells including carrier-carrier and carrier-phonon scattering and light propagation effects. The contributions of many-particle processes are nonadditive and thus cannot be treated separately. It is shown that due to nondiagonal correlation contributions, scattering rates alone cannot be taken as a measure for the dephasing of the intersubband polarization. Surprisingly, radiative damping is found to be important even at moderate carrier densities. Calculated absorption spectra are in excellent agreement with experiments on a high-quality sample.

We investigate the optical properties of a Coulomb-coupled double-quantum dot system excited by coherent light pulses. Basic effects of Coulomb coupling regarding linear and nonlinear optical processes are discussed. By numerically solving the Heisenberg equation of motion we are able to present the temporal evolution of the system's density matrix for a wide range of coupling parameters. The two main coupling effects in dipole approximation, biexcitonic shift and Förster energy transfer, are investigated and their qualitative and quantitative influence on absorption spectra, Rabi oscillations, and single-and two-pulse excitation is discussed. We present simulated differential transmission spectra to allow for comparison with recent experimental studies.

An important source of innovation in nanophotonics is the idea to scale down known radio wave technologies to the optical regime. One thoroughly investigated example of this approach are metallic nanoantennas which employ plasmonic resonances to couple localized emitters to selected far-field modes. While metals can be treated as perfect conductors in the microwave regime, their response becomes Drude-like at optical frequencies. Thus, plasmonic nanoantennas are inherently lossy. Moreover, their resonant nature requires precise control of the antenna geometry. A promising way to circumvent these problems is the use of broadband nanoantennas made from low-loss dielectric materials. Here, we report on highly directional emission from hybrid dielectric leaky-wave nanoantennas made of Hafnium dioxide nanostructures deposited on a glass substrate. Colloidal semiconductor quantum dots deposited in the nanoantenna feed gap serve as a local light source. The emission patterns of hybrid nanoantennas with different sizes are measured by Fourier imaging. We find for all antenna sizes a highly directional emission, underlining the broadband operation of our design.Nanoantennas have become valuable elements of the photonics toolbox to control and manipulate light on the nanoscale [1-3]. They allow for an efficient interconversion of localized excitations and propagating electromagnetic waves [4,5]. In receiving mode, nanoantennas can locally increase the light intensity by several orders of magnitude [6][7][8]. This property can be used for the efficient excitation of quantum emitters [9,10] and to boost nonlinear effects [11][12][13][14][15]. In transmitting mode, coupling of quantum emitters to nanoantennas allows for the control of the emission properties [16][17][18][19][20]. For instance, Curto et al reported on a highly directional plasmonic Yagi-Uda antenna [17] and Lee et al. demonstrated a planar dielectric antenna with near unity collection efficiency [20].Like their microwave counterparts, nanoantennas can be categorized based on their functional principle into two large groups: (i) resonant antennas and (ii) nonresonant traveling wave antennas. So far, most research has focused on resonant nanoantennas based either on plasmonic resonances in metals [18,[21][22][23] or on Mie resonances in highrefractive index dielectrics [24][25][26]. The latter offer the prospect of reducing dissipative losses while still providing large resonant enhancements of the electromagnetic near field. A recent review on optically resonant dielectric nanoantennas can be found in reference [27]. Moreover, dielectric antennas have been used in dielectric gradient metasurfaces as scattering elements [28]. In contrast to this, traveling wave antennas operating at optical frequencies have been studied considerably less. However, there is a growing interest in transferring the traveling wave concept to higher operating frequencies in order to achieve non-resonant broadband operation [29][30][31].Leaky-wave antennas are a subset of traveling wa...