We demonstrate the first emitter, based on a single optical source device, capable of addressing three species of interest (CO₂, CH₄, and H₂O) for differential absorption Lidar remote sensing of atmospheric greenhouse gases from space in the 2 μm region. It is based on an amplified nested cavity optical parametric oscillator. The single frequency source shows a total conversion efficiency of 37% and covers the 2.05-2.3 μm range.
We report on infrared quantum counting of photons at optical communication wavelengths based on nondegenerate two-photon absorption in a GaAs photomultiplier tube. The detected photon energy is lower than the GaAs band gap and the energy difference is complemented by a high intensity pump field. This detection setup is simple, compact, has a broad spectral bandwidth, and benefits from the intrinsic low noise and dark counts of large band gap semiconductor junctions.
We present novel frequency tuning methods for broadband mid-infrared spectroscopy that take advantage of the unique frequency sampling properties of our recently developed "nested dual-cavity doubly resonant optical parametric oscillator" (NesCOPO). These methods, referred to as Vernier frequency sampling, enable mode-hop tuning with an adjustable virtual-cavity intermode spacing. Both frequency resolution and span are widely adjustable and can be tailored to fulfill the requirements either for broadband spectroscopy (>50 cm −1 spectral coverage) at low resolution or for high resolution (<0.01 cm −1 ) narrow band spectroscopy. The technique is applied to short-range (10 to 30 m) atmospheric CO 2 measurements at 4.2 μm using integrated path differential absorption LIDAR.
We demonstrate a nanosecond single-frequency nested cavity optical parametric oscillator (NesCOPO) based on orientation-patterned GaAs (OP-GaAs). Its low threshold energy of 10 μJ enables to pump it with a pulsed single-frequency Tm:YAP microlaser. Stable single-longitudinal-mode emission is obtained owing to Vernier spectral filtering provided by the dual-cavity doubly-resonant NesCOPO scheme. Crystal temperature tuning covers the 10.3-10.9 μm range with a quasi-phase-matching period of 72.6 μm. A first step toward the implementation of this device in a differential absorption lidar is demonstrated by carrying out short-range standoff detection of ammonia vapor around 10.4 μm. Owing to the single-frequency emission, interferences due to absorption by atmospheric water vapor can be discriminated from the analyte signal.
We report on the capability of a direct detection differential absorption lidar (DIAL) for range resolved and integrated path (IPDIAL) remote sensing of CO in the atmospheric boundary layer (ABL). The laser source is an amplified nested cavity optical parametric oscillator (NesCOPO) emitting approximately 8 mJ at the two measurement wavelengths selected near 2050 nm. Direct detection atmospheric measurements are taken from the ground using a 30 Hz frequency switching between emitted wavelengths. Results show that comparable precision measurements are achieved in DIAL and IPDIAL modes (not better than a few ppm) on high SNR targets such as near range ABL aerosol and clouds, respectively. Instrumental limitations are analyzed and degradation due to cloud scattering variability is discussed to explain observed DIAL and IPDIAL limitations.
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