Rough or patterned surfaces infused with a lubricating liquid display many of the same useful properties as conventional gas-cushioned superhydrophobic surfaces. However, liquid-infused surfaces exhibit a new failure mode: the infused liquid film may drain due to an external shear flow, causing the surface to lose its advantageous properties. We examine shear-driven drainage of liquid-infused surfaces with the goal of understanding and thereby mitigating this failure mode. On patterned surfaces exposed to a known shear stress, we find that a finite length of the surface remains wetted indefinitely, despite the fact that no physical barriers prevent drainage. We develop an analytical model to explain our experimental results, and find that the steady-state retention results from the ability of patterned surfaces to wick wetting liquids, and is thus analogous to capillary rise. We establish the geometric surface parameters governing fluid retention and show how these parameters can describe even random substrate patterns.
We present a mathematical model and corresponding series of microfluidic experiments examining the flow of a viscous fluid past an elastic fibre in a three-dimensional channel. The fibre’s axis lies perpendicular to the direction of flow and its base is clamped to one wall of the channel; the sidewalls of the channel are close to the fibre, confining the flow. Experiments show that there is a linear relationship between deflection and flow rate for highly confined fibres at low flow rates, which inspires an asymptotic treatment of the problem in this regime. The three-dimensional problem is reduced to a two-dimensional model, consisting of Hele-Shaw flow past a barrier, with boundary conditions at the barrier that allow for the effects of flexibility and three-dimensional leakage. The analysis yields insight into the competing effects of flexion and leakage, and an analytical solution is derived for the leading-order pressure field corresponding to a slit that partially blocks a two-dimensional channel. The predictions of our model show favourable agreement with experimental results, allowing measurement of the fibre’s elasticity and the flow rate in the channel.
We present a co-flow microfluidic method to coat paramagnetic beads with a thin layer of fluid as the beads are pulled across a liquid-liquid interface by an external magnetic field. We show that the coating thickness can be controlled by the magnitude of the flow speed. Also, the number of beads aggregated within a single coating can be adjusted by varying the strength of the magnetic field or the liquid-liquid interfacial tension. V
When a pressurized fluid is injected into an elastic matrix, the fluid generates a fracture that grows along a plane and forms a fluid-filled disc-like shape. We report a laboratory study of such a fluid-driven crack in a gelatin matrix, study the crack shape as a function of time and investigate the influence of different experimental parameters such as the injection flow rate, Young’s modulus of the matrix and fluid viscosity. We choose parameters so that effects of material toughness are small. We find that the crack radius R ( t ) increases with time t according to t α with α =0.48±0.04. The rescaled experimental data at long times for different parameters collapse based on scaling arguments, available in the literature, showing R ( t )∝ t 4/9 from a balance of viscous stresses from flow along the crack and elastic stresses in the surrounding matrix. Also, we measure the time evolution of the crack shape, which has not been studied before. The rescaled crack shapes collapse at longer times and show good agreement with the scaling arguments. The gelatin system provides a useful laboratory model for further studies of fluid-driven cracks, which has important applications such as hydraulic fracturing.
Liquid-infused surfaces display advantageous properties that are normally associated with conventional gas-cushioned superhydrophobic surfaces. However, the surfaces can lose their novel properties if the infused liquid drains from the surface. We explore how drainage due to gravity or due to an external flow can be prevented through the use of chemical patterning. A small area of the overall surface is chemically treated to be preferentially wetted by the external fluid rather than the infused liquid. These sacrificial regions disrupt the continuity of the infused liquid, thereby preventing the liquid from draining from the texture. If the regions are patterned with the correct periodicity, drainage can be prevented entirely. The chemical patterns are created using spray-coating or deep-UV exposure, two facile techniques that are scalable to generate large-scale failure-resistant surfaces.
We describe a technique that measures ultralow interfacial tensions using paramagnetic spheres in a co-flow microfluidic device designed with a magnetic section. Our method involves tuning the distance between the co-flowing interface and the magnet's center, and observing the behavior of the spheres as they approach the liquid-liquid interface-the particles either pass through or are trapped by the interface. Using threshold values of the magnet-to-interface distance, we make estimates of the two-fluid interfacial tension. We demonstrate the effectiveness of this technique for measuring very low interfacial tensions, O(10(-6)-10(-5)) N m(-1), by testing solutions of different surfactant concentrations, and we show that our results are comparable with measurements made using a spinning drop tensiometer.
[1] One of the more distinctive features of many ignimbrites is the presence of large lithics (some greater than meter scale) and pumices that have been transported great distances (>10 km) from the eruptive vent, sometimes over steep terrain and expanses of water. In many cases, these particles have been transported much further than can be explained by aerodynamic forces and ballistic trajectories. We examine the forces responsible for transport of large clasts and examine in detail the momentum transfer occurring when particles interact with their boundaries. We performed a suite of experiments and numerical simulations to quantify the mass and momentum transfer that occurs when particles interact with a pumice bed substrate and with water substrate, two geologically motivated flow end-members. We find that clasts transported in dilute currents are particularly sensitive to the nature of the boundary, and while large particles can skip several times on a water substrate, they travel less far than particles that impact pumice bed substrates. All else being equal, large particles in dense pyroclastic density currents are themselves relatively insensitive to the details of their boundaries; however, one of the most important ways boundary conditions influence large particles is not through direct interaction but by changing the local concentration of fine particles. Momentum transfer from fine particles to large particles appears to be required to transport large clasts great distances. If initially dense flows become dilute during transport, then the transport capacity of large particles in the flow is substantially decreased.
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