We demonstrate the defect-free assembly of versatile target patterns of up 111 neutral atoms, building on a 361-site subset of a micro-optical architecture that readily provides thousands of sites for single-atom quantum systems. By performing multiple assembly cycles in rapid succession, we drastically increase achievable structure sizes and success probabilities. We implement repeated target pattern reconstruction after atom loss and deterministic transport of partial atom clusters necessary for distributing entanglement in large-scale systems. This technique will propel assembledatom architectures beyond the threshold of quantum advantage and into a regime with abundant applications in quantum sensing and metrology, Rydberg-state mediated quantum simulation, and error-corrected quantum computation.