Strategies toward ambitious climate targets usually rely on the concept of 'decoupling'; that is, they aim at promoting economic growth while reducing the use of natural resources and GHG emissions. GDP growth coinciding with absolute reductions in emissions or resource use is denoted as 'absolute decoupling' , as opposed to 'relative decoupling' , where resource use or emissions increase less so than does GDP. Based on the bibliometric mapping in part I (Wiedenhofer et al, 2020 Environ. Res. Lett. 15 063002), we synthesize the evidence emerging from the selected 835 peer-reviewed articles. We evaluate empirical studies of decoupling related to final/useful energy, exergy, use of material resources, as well as CO 2 and total GHG emissions. We find that relative decoupling is frequent for material use as well as GHG and CO 2 emissions but not for useful exergy, a quality-based measure of energy use. Primary energy can be decoupled from GDP largely to the extent to which the conversion of primary energy to useful exergy is improved. Examples of absolute long-term decoupling are rare, but recently some industrialized countries have decoupled GDP from both production-and, weaklier, consumption-based CO 2 emissions. We analyze policies or strategies in the decoupling literature by classifying them into three groups:(1) Green growth, if sufficient reductions of resource use or emissions were deemed possible without altering the growth trajectory.(2) Degrowth, if reductions of resource use or emissions were given priority over GDP growth. (3) Others, e.g. if the role of energy for GDP growth was analyzed without reference to climate change mitigation. We conclude that large rapid absolute reductions of resource use and GHG emissions cannot be achieved through observed decoupling rates, hence decoupling needs to be complemented by sufficiency-oriented strategies and strict enforcement of absolute reduction targets. More research is needed on interdependencies between wellbeing, resources and emissions.

As long as economic growth is a major political goal, decoupling growth from resource use and emissions is a prerequisite for a sustainable net-zero emissions future. However, empirical evidence for absolute decoupling, i.e. decreasing resource use and emissions at the required scale despite continued economic growth, is scarce and scattered across different research streams. In this two-part systematic review, we assess how and to what extent decoupling has been observed and what can be learnt for addressing the sustainability and climate crisis. Based on a transparent approach, we systematically identify and screen more than 11 500 scientific papers, eventually analyzing full texts of 835 empirical studies on the relationship between economic growth (GDP), resource use (materials and energy) and greenhouse gas emissions. Part I of the review examines how decoupling has been investigated across three research streams: energy, materials and energy, and emissions. Part II synthesizes the empirical evidence and policy implications (Haberl et al 2020 Environ. Res. Lett. 15 065003). In part I, we examine the topical, temporal and geographical scopes, methods of analysis, institutional networks and prevalent conceptual angles. We find that in this rapidly growing literature, the vast majority of studies-decomposition, 'causality' and Environmental Kuznets Curve analysis-approach the topic from a statistical-econometric point of view, while hardly acknowledging thermodynamic principles on the role of energy and materials for socio-economic activities. A potentially fundamental incompatibility between economic growth and systemic societal changes to address the climate crisis is rarely considered. We conclude that the existing wealth of empirical evidence merits braver conceptual advances than we have seen thus far. Future work should focus on comprehensive multi-indicator long-term analyses, conceptually grounded on the fundamental biophysical basis of socio-economic activities, incorporating the role of global supply chains as well as the wider societal role and preconditions of economic growth.

Dynamic material flow analysis (dMFA) is widely used to model stock‐flow dynamics. To appropriately represent material lifetimes, recycling potentials, and service provision, dMFA requires data about the allocation of economy‐wide material consumption to different end‐use products or sectors, that is, the different product stocks, in which material consumption accumulates. Previous estimates of this allocation only cover few years, countries, and product groups. Recently, several new methods for estimating end‐use product allocation in dMFA were proposed, which so far lack systematic comparison. We review and systematize five methods for tracing material consumption into end‐use products in inflow‐driven dMFA and discuss their strengths and limitations. Widely used data on industry shipments in physical units have low spatio‐temporal coverage, which limits their applicability across countries and years. Monetary input–output tables (MIOTs) are widely available and their economy‐wide coverage makes them a valuable source to approximate material end‐uses. We find four distinct MIOT‐based methods: consumption‐based, waste input–output MFA (WIO‐MFA), Ghosh absorbing Markov chain, and partial Ghosh. We show that when applied to a given MIOT, the methods’ underlying input–output models yield the same results, with the exception of the partial Ghosh method, which involves simplifications. For practical applications, the MIOT system boundary must be aligned to those of dMFA, which involves the removal of service flows, sector (dis)aggregation, and re‐defining specific intermediate outputs as final demand. Theoretically, WIO‐MFA, applied to a modified MIOT, produces the most accurate results as it excludes massless and waste transactions. In part 2 of this work, we compare methods empirically and suggest improvements for aligning MIOT‐dMFA system boundaries.

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Herein, a techno-economic and environmental performance evaluation (i.e. Life Cycle Assessment (LCA)) of a 45 kW Microbial Electrolysis Cell system is presented in the context of industrial wastewater conversion.