1T-TaS 2 is a charge-density-wave (CDW) compound with a Mott-insulating ground state. The metallic state obtained by doping, substitution or pulsed charge injection is characterized by an emergent CDW domain wall network, while single domain walls can be found in the pristine Mott state. Here we study whether and how the single walls become metallic. Tunneling spectroscopy reveals partial suppression of the Mott gap and the presence of in-gap states strongly localized at the domain-wall sites. Using the real-space dynamical mean field theory description of the strongly correlated quantum-paramagnet ground state we show that the local gap suppression follows from the increased hopping along the connected zigzag chain of lattice sites forming the domain wall, and that full metallisation is preempted by the splitting of the quasiparticle band into bonding and antibonding sub-bands due to the structural dimerization of the wall, explaining the presence of the in-gap states and the low density of states at the Fermi level.The interplay between superconductivity (SC) and correlated insulating phases, such as Mott insulators and charge density waves (CDW), is one of the central problems in condensed-matter physics. Remarkably, their combination can be found even in simple material systems, such as transition metal dichalcogenide (TMD) van der Waals compound 1T-TaS 2 . The ground state is a Mott insulator[1-3] with CDW[4] and unconventional quantum spin liquid behavior [5][6][7][8][9][10]. Upon Se substitution[11], Fe intercalation [12], or by applying pressure[13] it becomes superconducting, with both CDW and correlated behavior still present. Further control over electronic properties is possible through non-equilibrium charge injection via ultrafast optical or electrical pulses [14][15][16][17][18][19][20][21], which lead to drastic insulator to metastable metal transition. The long-standing hypothesis for metallisation and SC onset is linked to the formation of CDW domain walls, seen in multiple TMDs with different techniques [22][23][24]. Recently, it was challenged experimentally with scanning tunneling spectroscopy (STS) [25], which showed the absence of metallisation in certain types of walls. First-principles calculations revealed that atomic reconstruction in the walls may cause the formation of bound states[25] and band reconstruction [24], but the correlation effects were left out of scope. Thus, the crucial question of whether the CDW distortion inside the wall can lead to Mottness collapse remains open. In this paper we combine STS and dynamical mean field theory (DMFT) calculations to study the behavior of the Mott gap in CDW domain walls, finding Mottness collapse without metallisation.In 1T-TaS 2 , each layer is periodically modulated to form a √ 13 × √ 13 superlattice of David star deformations [4], resulting in a commensurate CDW state with a single half-filled electron band at the Fermi level [26,27]. The Coulomb repulsion opens a charge gap in this band, resulting in a Mott insulating ground state [2...
The interplay between local, repulsive interactions and disorder acting only on one spin orientation of lattice fermions ("spin-dependent disorder") is investigated. The nonmagnetic disorder vs. interaction phase diagram is computed using Dynamical Mean-Field Theory in combination with the geometric average over disorder. The latter determines the typical local density of states and is therefore sensitive to Anderson localization. The effect of spin-dependent disorder is found to be very different from that of conventional disorder. In particular, it destabilizes the metallic solution and leads to a novel spin-selective, localized phase at weak interactions and strong disorder.
Motivated by the rapidly growing possibilities for experiments with ultracold atoms in optical lattices, we investigate the thermodynamic properties of correlated lattice fermions in the presence of an external spindependent random potential. The corresponding model, a Hubbard model with spin-dependent local random potentials, is solved within dynamical mean-field theory. This allows us to present a comprehensive picture of the thermodynamic properties of this system. In particular, we show that for a fixed total number of fermions spin-dependent disorder induces a magnetic polarization. The magnetic response of the polarized system differs from that of a system with conventional disorder.
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