Thermoplastic composites containing different Ground Rubber Tire (GRT) materials, Linear Low Density Polyethylene (LLDPE) and, in some case, a coupling agent (IB‘E’, an ethylene glycidyl methacrylate copolymer) were prepared by melt blending. The impact energies of all the thermoplastic composites (normally containing 40 wt % GRT) were evaluated using an instrumented impact tester. The effects of the GRT particle-size, particle size distribution and shape, the mode of grinding, and the oxygen surface concentration were analyzed. The wet-ambient-ground GRT based composites show higher surface oxidation and give better impact energy than cryo-ground and normal air-ground GRT based composites. Smaller GRT particle size results in a small increase in the impact property of the composite and a greater influence on the melt processability of the composites. Of the different GRT surface modification techniques studied for improved composite interfacial adhesion and impact properties the composites from electron beam radiation treated GRT yield higher increases in impact energy in comparison to corona and plasma treated GRT based composites.
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