A long-standing prediction of nuclear models is the emergence of a region of long-lived, or even stable, superheavy elements beyond the actinides. These nuclei owe their enhanced stability to closed shells in the structure of both protons and neutrons. However, theoretical approaches to date do not yield consistent predictions of the precise limits of the 'island of stability'; experimental studies are therefore crucial. The bulk of experimental effort so far has been focused on the direct creation of superheavy elements in heavy ion fusion reactions, leading to the production of elements up to proton number Z = 118 (refs 4, 5). Recently, it has become possible to make detailed spectroscopic studies of nuclei beyond fermium (Z = 100), with the aim of understanding the underlying single-particle structure of superheavy elements. Here we report such a study of the nobelium isotope 254No, with 102 protons and 152 neutrons--the heaviest nucleus studied in this manner to date. We find three excited structures, two of which are isomeric (metastable). One of these structures is firmly assigned to a two-proton excitation. These states are highly significant as their location is sensitive to single-particle levels above the gap in shell energies predicted at Z = 114, and thus provide a microscopic benchmark for nuclear models of the superheavy elements.

Abstract. The odd-Z isotope

Lifetimes of prolate intruder states in 186Pb and oblate intruder states in 194Po have been determined by employing, for the first time, the recoil-decay tagging technique in recoil distance Doppler-shift lifetime measurements. In addition, lifetime measurements of prolate states in 188Pb up to the 8+ state were carried out using the recoil-gating method. The B(E2) values have been deduced from which deformation parameters |beta2|=0.29(5) and |beta2|=0.17(3) for the prolate and the oblate bands, respectively, have been extracted. The results also shed new light on the mixing between different shapes.

Lifetimes of yrast states in 180 Hg up to the 8 + state and of the 9 − state have been extracted from recoil-decay tagged γ -ray spectra by using the recoil distance Doppler-shift method. In addition, lifetimes of yrast states up to the 10 + state in 182 Hg have been extracted from recoil-gated γ γ -coincidence spectra. The present study addresses the evolution of collectivity of two competing shapes in neutron-deficient Hg nuclei as a function of A and the configuration mixing at low spin.

No abstract

No abstract

No abstract

Using fusion-evaporation reactions, a gas-filled recoil separator, and recoil-electron and recoil-electron-α tagging techniques, a new isomeric 1 2 201 At is identified, and an earlier reported corresponding state [T 1/2 = 273( 9) ms] in 199 At is confirmed. The 1 2 + state is suggested to originate from an intruder π (s 1/2 ) −1 configuration. In addition, nuclear structure of states below and above this 1 2 + state are studied in both nuclei. The isomer decays through a cascade of an E3 transition followed by a mixed M1/E2 transition to the 9 2 − ground state, and it is interpreted to be fed from nearly spherical 3 2 + and 5 2 + states originating from π (d 3/2 ) −1 and π (d 5/2 ) −1 configurations, respectively.