Superconductivity and ferromagnetism are two mutually antagonistic states in condensed matter. Research on the interplay between these two competing orderings sheds light not only on the cause of various quantum phenomena in strongly correlated systems but also on the general mechanism of superconductivity. Here we report on the observation of the electronic entanglement between superconducting and ferromagnetic states in hydrogenated boron-doped nanodiamond films, which have a superconducting transition temperature T ∼ 3 K and a Curie temperature T > 400 K. In spite of the high T, our nanodiamond films demonstrate a decrease in the temperature dependence of magnetization below 100 K, in correspondence to an increase in the temperature dependence of resistivity. These anomalous magnetic and electrical transport properties reveal the presence of an intriguing precursor phase, in which spin fluctuations intervene as a result of the interplay between the two antagonistic states. Furthermore, the observations of high-temperature ferromagnetism, giant positive magnetoresistance, and anomalous Hall effect bring attention to the potential applications of our superconducting ferromagnetic nanodiamond films in magnetoelectronics, spintronics, and magnetic field sensing.
Recent progress in neutron spin-echo spectroscopy by means of longitudinal Modulation of IntEnsity with Zero Effort (MIEZE) is reviewed. Key technical characteristics are summarized which highlight that the parameter range accessible in momentum and energy, as well as its limitations, are extremely well understood and controlled. Typical experimental data comprising quasi-elastic and inelastic scattering are presented, featuring magneto-elastic coupling and crystal field excitations in Ho 2 Ti 2 O 7 , the skyrmion lattice to paramagnetic transition under applied magnetic field in MnSi, ferromagnetic criticality and spin waves in Fe. In addition bench marking studies of the molecular dynamics in H 2 O are reported. Taken together, the advantages of MIEZE spectroscopy in studies at small and intermediate momentum transfers comprise an exceptionally wide dynamic range of over seven orders of magnitude, the capability to perform straight forward studies on depolarizing samples or under depolarizing sample environments, as well as on incoherently scattering materials.
Magnetic nanoparticles offer unique potential for various technological, biomedical, or environmental applications thanks to the size-, shape- and material-dependent tunability of their magnetic properties. To optimize particles for a specific...
The instrumental layout and technical realisation of the neutron resonant spin echo (NRSE) spectrometer RESEDA at the Heinz Maier-Leibnitz Zentrum (MLZ) in Garching, Germany, is presented. RESEDA is based on a longitudinal field configuration, boosting both dynamic range and maximum resolution of the spectrometer compared to the conventional transverse layout. The resonant spin echo technique enables the realisation of two complementary techniques: A longitudinal NRSE (LNRSE) option comparable to the classical neutron spin echo (NSE) method for highest energy resolution and large momentum transfers as well as a Modulation of Intensity with Zero Effort (MIEZE) option for depolarising samples or sample environments such as high magnetic fields, and strong incoherent scattering samples. With their outstanding dynamic range, exceeding nominally seven orders of magnitude, both options cover new fields for ultra-high resolution neutron spectroscopy in hard and soft condensed matter systems. In this paper the concept of RESEDA as well as the technical realisation along with reference measurements are reported.
The generation of high frequency oscillatory magnetic fields represents a fundamental component underlying the successful implementation of neutron resonant spin-echo spectrometers, a class of instrumentation critical for the high-resolution extraction of dynamical excitations (structural and magnetic) in materials. In this paper, the setup of the resonant circuits at the longitudinal resonant spin-echo spectrometer RESEDA is described in comprehensive technical detail. We demonstrate that these circuits are capable of functioning at frequencies up to 3.6 MHz and over a broad bandwidth down to 35 kHz using a combination of signal generators, amplifiers, impedance matching transformers, and a carefully designed cascade of tunable capacitors and customized coils.
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