This study examines the vertical variations of cloud microphysical relationships and their implications to cloud microphysical processes in marine stratocumulus clouds using in‐situ aircraft observations during the Aerosol and Cloud Experiments in Eastern North Atlantic (ACE‐ENA) field campaign. A new diagram with a coordinate system based on cloud droplet liquid water content (Lc) and phase relaxation time scale is proposed to investigate mixing mechanisms. This new diagram analysis shows that the inhomogeneous mixing trait is dominant near the cloud top, but homogeneous mixing trait is stronger at lower altitudes. The relevant scale parameters (i.e., transition length scale and transition scale number) also indicate a high likelihood of inhomogeneous mixing. The relationship between Lc and standard deviation of droplet radius (σR) clearly shows the vertical transition: the correlation between Lc and σR is positive at lower cloud altitudes, but it becomes negative as altitude increases. Such a vertical transition is consistent with the vertical circulation mixing, modulating the cloud microphysical relationships to suggest homogeneous mixing at a significant depth from the cloud top.

To enhance our understanding of fog processes over complex terrain, various fog events that occurred during the International Collaborative Experiments for Pyeongchang 2018 Winter Olympics and Paralympics (ICE-POP) campaign were selected. Investigation of thermodynamic, dynamic, and microphysical conditions within fog layers affected by quasi-periodic oscillation of atmospheric variables was conducted using observations from a Fog Monitor-120 (FM-120) and other in-situ meteorological instruments. A total of nine radiation fog cases that occurred in the autumn and winter seasons during the campaign over the mountainous region of Pyeongchang, Korea were selected. The wavelet analysis was used to study quasi-period oscillations of dynamic, microphysical, and thermodynamic variables. By decomposing the time series into the time-frequency space, we can determine both dominant periods and how these dominant periods change in time. Quasi-period oscillations of liquid water content (LWC), pressure, temperature, and horizontal/vertical velocity, which have periods of 15–40 min, were observed during the fog formation stages. We hypothesize that these quasi-periodic oscillations were induced by Kelvin–Helmholtz instability. The results suggest that Kelvin–Helmholtz instability events near the surface can be explained by an increase in the vertical shear of horizontal wind and by a simultaneous increase in wind speed when fog forms. In the mature stages, fluctuations of the variables did not appear near the surface anymore.

Cloud microphysical relationships observed during the Cloud System Evolution in the Trades (CSET) campaign held between Northern California and Hawaii were analyzed to study the effects of entrainment and subsequent mixing of free-tropospheric and cloudy air on cloud microphysical properties of marine stratocumulus clouds. The data measured by Holographic Detector for Clouds (HOLODEC) were extensively used because they could provide the 3D positions and sizes of droplets within sample volume on the centimeter scale, making it possible to explore the 3D spatial distribution of droplets, which has not been possible for conventional cloud probes. This study focused on analyzing the 3D spatial distribution of droplets and visual traits of inhomogeneous mixing and on quantifying the relationship between 3D spatial distributions and traits of inhomogeneous mixing. Two types of spatial distributions are compared. The first is measured droplet spatial distribution and the second type is generated randomly distributed droplets using the Monte Carlo approach, that is, to analyze whether or not clustering is strong enough to classify as a clustered distribution for a hologram. The difference between the two types of spatial distributions depends on whether they are affected by entrainment and mixing. The holograms observed near the cloud top, where the effects of entrainment and mixing would be immediate, showed relatively high confidence in the significance test for spatially clustered populations of droplets. Moreover, spatially clustered holograms appeared to exhibit stronger visual traits of inhomogeneous mixing than perfectly randomly distributed holograms only when observed near the cloud top. On the other hand, these characteristics did not appear for holograms observed deeper into the cloud where the effects of entrainment and mixing would be reduced. Such 3D structural characteristics of droplet distributions seem to be consistent with vertical circulation mixing.