Composite magnetic particles (CMP) with carbonyl iron (CI) core and poly (methyl methacrylate) shell were prepared by an in-situ dispersion polymerization method via surface treated CI with acrylic acid. These CMP were adopted as dispersed phase of magnetorheological (MR) fluids, and has better MR fluids characteristics than fluid with CI alone as they have severe sedimentation and poor dispersion quality. Flow properties of the MR fluids were analyzed via a rotational rheometer equipped with a magnetic field supplier in parallel plate geometry.Index Terms-Carbonyl iron, composite, magnetorheological fluid, poly (methyl methacrylate) (PMMA).

Carbonyl iron ͑CI͒ has been widely used as a suspended particle in magnetorheological ͑MR͒ fluids. However, pristine CI-based MR fluids have several drawbacks, including severe sedimentation of the CI particles due to the large density difference with the carrier liquid, difficulties in redispersion after caking, abrasion of device surfaces during long-term operation, and rust of iron by oxidation. To overcome these shortcomings, we coated the CI particles with a poly͑vinyl butyral͒ ͑PVB͒ shell. CI and CI-PVB particles were suspended in mineral oil and their MR characteristics were examined via a rotational rheometer in a parallel plate geometry equipped with a magnetic field supplier. Yield stress and flow response ͑shear stress and shear viscosity͒ were investigated at magnetic field strengths ranging from 0 to 343 kA/ m. Although the MR properties, such as yield stress and shear viscosity of CI-PVB based MR fluids, changed slightly compared with those of the pristine CI based MR fluid, the dispersion qualities ͑e.g., sedimentation stability͒ were noticeably improved.

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