Conductive films that are both stretchable and flexible could have applications in electronic devices, sensors, actuators and speakers. A substantial amount of research has been carried out on conductive polymer composites, metal electrode-integrated rubber substrates and materials based on carbon nanotubes and graphene. Here we present highly conductive, printable and stretchable hybrid composites composed of micrometre-sized silver flakes and multiwalled carbon nanotubes decorated with self-assembled silver nanoparticles. The nanotubes were used as one-dimensional, flexible and conductive scaffolds to construct effective electrical networks among the silver flakes. The nanocomposites, which included polyvinylidenefluoride copolymer, were created with a hot-rolling technique, and the maximum conductivities of the hybrid silver-nanotube composites were 5,710 S cm⁻¹ at 0% strain and 20 S cm⁻¹ at 140% strain, at which point the film ruptured. Three-dimensional percolation theory reveals that Poisson's ratio for the composite is a key parameter in determining how the conductivity changes upon stretching.
The annelid provides a biological solution of effective locomotion adaptable to a large variety of unstructured environmental conditions. The undulated locomotion of the segmented body in the annelid is characterized by the combination of individual motion of the muscles distributed along the body, which has been of keen interest in biomimetic investigation. In this paper, we present an annelid-like robot driven by soft actuators based on dielectric elastomer. To mimic the unique motion of the annelid, a novel actuation method employing dielectric elastomer is developed. By using the actuator, a three-degree-of-freedom actuator module is presented, which can provide up-down translational motion, and two rotational degree-of-freedom motion. The proposed actuation method provides advantageous features of reduction in size, fast response and ruggedness in operation. By serially connecting the actuator modules, a micro-robot mimicking the motion of the annelid is developed and its effectiveness is experimentally demonstrated.
An adhesive with high conductivity, flexibility, cyclability, oxidation resistance, and good adhesion is developed using microscale silver flakes, multiwalled carbon nanotubes decorated with nanoscale silver particles, and nitrile butadiene rubber. Light-emitting-diode chips are attached to the conductive, flexible adhesive pattern on a poly(ethylene terephthalate) substrate as a visual demonstration. The brightness is invariant during bending tests.
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