It has long been speculated that electronic flatband systems can be a fertile ground for hosting novel emergent phenomena including unconventional magnetism and superconductivity 1-14 . Here we use scanning tunnelling microscopy to elucidate the atomically resolved electronic states and their magnetic response in the kagome magnet 15-20 Co3Sn2S2. We observe a pronounced peak at the Fermi level, which is identified to arise from the kinetically frustrated kagome flatband. Increasing magnetic field up to ±8T, this state exhibits an anomalous magnetization-polarized Zeeman shift, dominated by an orbital moment in opposite to the field direction. Such negative magnetism can be understood as spin-orbit coupling induced quantum phase effects 21-25 tied to non-trivial flatband systems. We image the flatband peak, resolve the associated negative magnetism, and provide its connection to the Berry curvature field, showing that Co3Sn2S2 is a rare example of kagome magnet where the low energy physics can be dominated by the spinorbit coupled flatband. Our methodology of probing band-resolved ordering phenomena such as spin-orbit magnetism can also be applied in future experiments to elucidate other exotic phenomena including flatband superconductivity and anomalous quantum transport.
Magnetic topological phases of quantum matter are an emerging frontier in physics and material science [1][2][3][4]. Along these lines, several kagome magnets [5][6][7][8][9] have appeared as the most promising platforms. However, the magnetic nature of these materials in the presence of topological state remains an unsolved issue [5][6][7][8][9]. Here, we explore magnetic correlations in the kagome magnet Co 3 Sn 2 S 2 . Using muon spin-rotation, we present evidence for competing magnetic orders in the kagome lattice of this compound. Our results show that while the sample exhibits an outof-plane ferromagnetic ground state, an in-plane antiferromagnetic state appears at temperatures above 90 K, eventually attaining a volume fraction of 80% around 170 K, before reaching a nonmagnetic state. Strikingly, the reduction of the anomalous Hall conductivity above 90 K linearly follows the disappearance of the volume fraction of the ferromagnetic state. We further show that the competition of these magnetic phases is tunable through applying either an external magnetic field or hydrostatic pressure. Our results taken together suggest the thermal and quantum tuning of Berry curvature field via external tuning of magnetic order. Our study shows that Co 3 Sn 2 S 2 is a rare example where the magnetic competition drives the thermodynamic evolution * Electronic address: zurab.guguchia@psi.ch of the Berry curvature field, thus tuning its topological state.The kagome lattice is a two-dimensional pattern of corner-sharing triangles. With this unusual symmetry and the associated geometrical frustration, the kagome lattice can host peculiar states including flat bands [8], Dirac fermions [5,6] and spin liquid phases [7,10]. In particular, magnetic kagome materials offer a fertile ground to study emergent behaviors resulting from the interplay between unconventional magnetism and band topology. Recently, transition-metal based kagome magnets [5][6][7][8][9][10][11][12][13] are emerging as outstanding candidates for such studies, as they feature both large Berry curvature fields and unusual magnetic tunability. In this family, the kagome magnet Co 3 Sn 2 S 2 is found to exhibit both a large anomalous Hall effect and anomalous Hall angle, and is identified as a promising Weyl semimetal candidate [9,11,14,15]. However, despite knowing the magnetic ground state is ferromagnetic below T C = 177 K [16] with spins aligned along the c-axis [9, 11, 17] (see Figs. 1 a and b) there is no report of its magnetic tunability or phase diagram, and its interplay with the topological band structure. Here we use high-resolution µSR to systematically characterize the phase diagram, uncovering another intriguing in-plane antiferromagnetic phase. The magnetic competition between these two phases is further found to be highly tunable via applying either pressure [18][19][20][21] or magnetic field. Combined with first principles calculations, we discover that the tunable magnetic correlation plays a key role in determining the giant anomalous Hall transp...
Charge density wave (CDW) is a startling quantum phenomenon, distorting a metallic lattice into an insulating state with a periodically modulated charge distribution. Astonishingly, such modulations appear in various patterns even within the same family of materials. Moreover, this phenomenon features a puzzling diversity in its dimensional evolution. Here, we propose a general framework, unifying distinct trends of CDW ordering in an isoelectronic group of materials, 2H-MX 2 (M = Nb, Ta and X = S, Se). We show that while NbSe 2 exhibits a strongly enhanced CDW order in two dimensions, TaSe 2 and TaS 2 behave oppositely, with CDW being absent in NbS 2 entirely. Such a disparity is demonstrated to arise from a competition of ionic charge transfer, electron-phonon coupling, and electron correlation. Despite its simplicity, our approach can, in principle, explain dimensional dependence of CDW in any material, thereby shedding new light on this intriguing quantum phenomenon and its underlying mechanisms.
A 1T-TaS2 CDW system offers ultrabroadband and high photosensitivity from visible to terahertz wavelengths at room temperature.
Exploration of the topological quantum materials with electron correlation is at the frontier of physics, as the strong interaction may give rise to new topological phases and transitions. Here we report that a family of kagome magnets RMn 6 Sn 6 manifest the quantum transport properties analogical to those in the quantum-limit Chern magnet TbMn 6 Sn 6 . The topological transport in the family, including quantum oscillations with nontrivial Berry phase and large anomalous Hall effect arising from Berry curvature field, points to the existence of Chern gapped Dirac fermions. Our observation demonstrates a close relationship between rare-earth magnetism and topological electron structure, indicating the rare-earth elements can effectively engineer the Chern quantum phase in kagome magnets.
We study the anomalous Hall effect (AHE) of single-crystalline Co 3 Sn 2−x In x S 2 over a large range of indium concentration x from 0 to 1. Their magnetization reduces progressively with increasing x while their ground state evolves from a ferromagnetic Weyl semimetal into a nonmagnetic insulator. Remarkably, after systematically scaling the AHE, we find that their intrinsic anomalous Hall conductivity (AHC) features an unexpected maximum at around x = 0.15. The change of the intrinsic AHC corresponds with the doping evolution of Berry curvature and the maximum arises from the magnetic topological nodal-ring gap. Our experimental results show a larger AHC in a fundamental nodal-ring gap than that of Weyl nodes.
Background: With the improvement of anesthesia and surgical techniques, supraglottic device with assist ventilation under general anesthesia (GA) combined with nerve block is gradually applied to video-assisted thoracoscopic surgery. However, the safety of assist ventilation has not been fully confirmed, and a large number of samples should be studied in clinical exploration. Methods: The subjects included 120 patients, undergoing elective thoracoscopic GA, with American Society of Anesthesiologists (ASA) physical status I or II, were randomly divided into 3 groups, 40 cases in each group. Group T: received double-lumen bronchial intubation, Group I: received intercostal nerve block using a supraglottic device, Group P: received paravertebral nerve block using a supraglottic device. Mean arterial pressure, heart rate, saturation of pulse oximetry and surgical field satisfaction, general anesthetic dosage and recovery time were recorded before induction of GA (T 0 ), at the start of the surgical procedure (T 1 ), 15 minutes later (T 2 ), 30 minutes later (T 3 ), and before the end of the surgical procedure (T 4 ). Static and dynamic pain rating (NRS) and Ramsay sedation score were recorded 2 hours after surgery (T 5 ), 12 hours after surgery (T 6 ), 24 hours after surgery (T 7 ), time to get out of bed, hospitalization time and cost, patient satisfaction and adverse reactions. Results: There was no significant difference with the surgical visual field of the 3 groups ( P > .05). The MAP, HR and SpO 2 of the 3 groups were decreased from T 2 to T 3 compared with T 0 ( P < .05). Compared with group T: the total dosage of GA was reduced in group I and group P, the recovery time was shorter, the time to get out of bed was earlier ( P < .05), the hospitalization time was shortened, the hospitalization cost was lower, and the patient satisfaction was higher ( P < .05). The static and dynamic NRS scores were lower from T 5 to T 7 ( P < .05). Ramsay sedation scores were higher ( P < .05), and the incidence of adverse reactions was lower ( P < .05). Comparison between group I and group P: Dynamic NRS score of group P was lower from T 6 to T 7 ( P < .05). Conclusion: ...
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