The helicopter-borne instrument payload known as the Airborne Cloud Turbulence Observation System (ACTOS) was used to study the entrainment and mixing processes in shallow warm cumulus clouds. The characteristics of the mixing process are determined by the Damkö hler number, defined as the ratio of the mixing and a thermodynamic reaction time scale. The definition of the reaction time scale is refined by investigating the relationship between the droplet evaporation time and the phase relaxation time. Following arguments of classical turbulence theory, it is concluded that the description of the mixing process through a single Damkö hler number is not sufficient and instead the concept of a transition length scale is introduced. The transition length scale separates the inertial subrange into a range of length scales for which mixing between ambient dry and cloudy air is inhomogeneous, and a range for which the mixing is homogeneous. The new concept is tested on the ACTOS dataset. The effect of entrained subsaturated air on the droplet number size distribution is analyzed using mixing diagrams correlating droplet number concentration and droplet size. The data suggest that homogeneous mixing is more likely to occur in the vicinity of the cloud core, whereas inhomogeneous mixing dominates in more diluted cloud regions. Paluch diagrams are used to support this hypothesis. The observations suggest that homogeneous mixing is favored when the transition length scale exceeds approximately 10 cm. Evidence was found that suggests that under certain conditions mixing can lead to enhanced droplet growth such that the largest droplets are found in the most diluted cloud regions. * Deceased.

Abstract. In this paper we describe and summarize the main achievements of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). EUCAARI started on 1 January 2007 and ended on 31 December 2010 leaving a rich legacy including: (a) a comprehensive database with a year of observations of the physical, chemical and optical properties of aerosol particles over Europe, (b) comprehensive aerosol measurements in four developing countries, (c) a database of airborne measurements of aerosols and clouds over Europe during May 2008, (d) comprehensive modeling tools to study aerosol processes fron nano to global scale and their effects on climate and air quality. In addition a new Pan-European aerosol emissions inventory was developed and evaluated, a new cluster spectrometer was built and tested in the field and several new aerosol parameterizations and computations modules for chemical transport and global climate models were developed and evaluated. These achievements and related studies have substantially improved our understanding and reduced the uncertainties of aerosol radiative forcing and air quality-climate interactions. The EUCAARI results can be utilized in European and global environmental policy to assess the aerosol impacts and the corresponding abatement strategies.

Clouds play an important role in Arctic amplification. This term represents the recently observed enhanced warming of the Arctic relative to the global increase of near-surface air temperature. However, there are still important knowledge gaps regarding the interplay between Arctic clouds and aerosol particles, and surface properties, as well as turbulent and radiative fluxes that inhibit accurate model simulations of clouds in the Arctic climate system. In an attempt to resolve this so-called Arctic cloud puzzle, two comprehensive and closely coordinated field studies were conducted: the Arctic Cloud Observations Using Airborne Measurements during Polar Day (ACLOUD) aircraft campaign and the Physical Feedbacks of Arctic Boundary Layer, Sea Ice, Cloud and Aerosol (PASCAL) ice breaker expedition. Both observational studies were performed in the framework of the German Arctic Amplification: Climate Relevant Atmospheric and Surface Processes, and Feedback Mechanisms (AC) project. They took place in the vicinity of Svalbard, Norway, in May and June 2017. ACLOUD and PASCAL explored four pieces of the Arctic cloud puzzle: cloud properties, aerosol impact on clouds, atmospheric radiation, and turbulent dynamical processes. The two instrumented Polar 5 and Polar 6 aircraft; the icebreaker Research Vessel (R/V) Polarstern; an ice floe camp including an instrumented tethered balloon; and the permanent ground-based measurement station at Ny-Ålesund, Svalbard, were employed to observe Arctic low- and mid-level mixed-phase clouds and to investigate related atmospheric and surface processes. The Polar 5 aircraft served as a remote sensing observatory examining the clouds from above by downward-looking sensors; the Polar 6 aircraft operated as a flying in situ measurement laboratory sampling inside and below the clouds. Most of the collocated Polar 5/6 flights were conducted either above the R/V Polarstern or over the Ny-Ålesund station, both of which monitored the clouds from below using similar but upward-looking remote sensing techniques as the Polar 5 aircraft. Several of the flights were carried out underneath collocated satellite tracks. The paper motivates the scientific objectives of the ACLOUD/PASCAL observations and describes the measured quantities, retrieved parameters, and the applied complementary instrumentation. Furthermore, it discusses selected measurement results and poses critical research questions to be answered in future papers analyzing the data from the two field campaigns.

On time scales that are long compared to the phase relaxation time, a quasi-steady supersaturation sqs is expected to exist in clouds. On shorter time scales, however, turbulent fluctuations of temperature and water vapor concentration should generate fluctuations in supersaturation. The variability of temperature, water vapor, and supersaturation has been measured in situ with submeter resolution in warm, continental, shallow cumulus clouds. Several cumuli with horizontal extents of order 100 m were sampled during their first appearance and development to depths of ~100 m in a growing boundary layer. Fluctuations of the saturation ratio are observed to be approximately normally distributed with standard deviations on the order of 1%. This variability is almost one order of magnitude larger than sqs calculated using simultaneous measurements of the vertical velocity component and the droplet size distribution. It is argued that, depending on the ratio of the phase relaxation and the turbulent mixing time, substantial fluctuations in the supersaturation field can exist on small spatial scales, centered on sqs for the mean state. The observations also suggest that, on larger scales, fluctuations of the supersaturation field are damped by cloud droplet growth. Droplets with diameters of up to 20 μm were observed in the shallow cumulus clouds, whereas the adiabatic diameter was less than 10 μm. Such large droplets may be explained by a few droplets experiencing the highest observed supersaturations for a certain time. Consequences for aerosol activation and droplet size dispersion in a highly fluctuating supersaturation field are briefly discussed.

A new helicopter payload designed to overcome rotor downwash allows better than 10 cm resolution for turbulence and microphysical observations in boundary layer clouds.

High-resolution measurements of the turbulent, thermodynamic, and microphysical structure of the edges of trade wind cumuli have been performed with the Airborne Cloud Turbulence Observation System. Lateral entrainment of subsaturated air into the cloud region leads to an evaporative cooling effect. The negatively buoyant air partly enhances the compensating downdraft, forming a subsiding shell at cloud edge. Based on the presented observations, the subsiding shell is divided into a turbulent and humid inner shell adjacent to the cloud interior and a nonbuoyant, nonturbulent outer shell. In the trade wind region, continuous development of shallow cumuli over the day allows for an analysis of the properties of both shells as a function of different cloud evolution stages. The shallow cumuli are divided into actively growing, decelerated, and dissolving based on cloud properties. As the cumuli evolve from actively growing to dissolving, the subsaturated environmental air is mixed deeper and deeper into the cloud region and the subsiding shell grows at the expense of the cloud. This measured evolution of the subsiding shell compares favorably with the predictions of a direct numerical simulation of an idealized subsiding shell. The thickness of the measured outer shell decreases with the evolution of the cumuli while the intensity of the downdraft is nearly constant.

Tethered balloon–borne measurements with a resolution in the order of 10 cm in a cloudy boundary layer are presented. Two examples sampled under different conditions concerning the clouds' stage of life are discussed. The hypothesis tested here is that basic ideas of classical turbulence theory in boundary layer clouds are valid even to the decimeter scale. Power spectral densities S( f ) of air temperature, liquid water content, and wind velocity components show an inertial subrange behavior down to ≈20 cm. The mean energy dissipation rates are ∼10−3 m2 s−3 for both datasets. Estimated Taylor Reynolds numbers (Reλ) are ∼104, which indicates the turbulence is fully developed. The ratios between longitudinal and transversal S( f ) converge to a value close to 4/3, which is predicted by classical turbulence theory for local isotropic conditions. Probability density functions (PDFs) of wind velocity increments Δu are derived. The PDFs show significant deviations from a Gaussian distribution with longer tails typical for an intermittent flow. Local energy dissipation rates ɛτ are derived from subsequences with a duration of τ = 1 s. With a mean horizontal wind velocity of 8 m s−1, τ corresponds to a spatial scale of 8 m. The PDFs of ɛτ can be well approximated with a lognormal distribution that agrees with classical theory. Maximum values of ɛτ ≈ 10−1 m2 s−3 are found in the analyzed clouds. The consequences of this wide range of ɛτ values for particle–turbulence interaction are discussed.

Abstract. Aerosol particle measurements in the atmospheric boundary layer performed by a helicopter-borne measurement payload and by a lidar system from a case study during the IMPACT field campaign in Cabauw (NL) are presented. Layers of increased number concentrations of ultrafine particles were observed in the residual layer, indicating relatively recent new-particle formation. These layers were characterized by a sub-critical Richardson number and concomitant increased turbulence. Turbulent mixing is likely to lead to local supersaturation of possible precursor gases which are essential for new particle formation. Observed peaks in the number concentrations of ultrafine particles at ground level are connected to the new particle formation in the residual layer by boundary layer development and vertical mixing.