Abstract. The horizontal distribution of radioactive cesium (Cs) derived from the Fukushima Dai-ichi nuclear power plant (FNPP) in the North Pacific is still unclear due to the limitation of direct measurement of the seawater in the open ocean. We present the result of direct observation of radioactive Cs in surface seawater collected from a broad area in the western and central North Pacific in July 2011, October 2011 and July 2012. We also conducted a simple particle tracking experiment to estimate the qualitative spatial distribution of radioactive Cs in the North Pacific. 134Cs was detected at 94 stations out of 123 stations, and 137Cs was detected at all stations. High 134Cs and 137Cs concentrations more than 10 m Bq kg−1 were observed in the area of the northern part of Kuroshio Extension at 144° E and 155° E in July 2011, in the area 147–175° E around 40° N in October 2011, and the northern part of Kuroshio Extension at 155° E and 175°30´ E in July 2012. Combining the result of direct observations and particle tracking experiment, the radioactive Cs derived from the FNPP had been dispersed eastward to the central North Pacific during 2011. It was considered from the horizontal distribution that radioactive Cs was dispersed not only eastward but also north- and southward in the central North Pacific. Pronounced dilution process of radioactive Cs from the FNPP during study period is suggested from temporal change in the activity ratio of 134Cs / 137Cs, which was decay-corrected on 6 April 2011, and relationships between radioactive Cs and temperature.

The spatial distributions of radiocesium concentration in sea sediment to a core depth of 14 cm were investigated in the offshore region from the Fukushima Prefecture to the northern part of the Ibaraki Prefecture in February and July 2012, at a spatial resolution of 5 min of latitude and longitude. The concentrations in the area south of the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) were generally higher than those in the area north of it. In the southern area, a band of especially high concentration with a width about 20 km was present in the region shallower than 100 m, and a narrow minimal concentration band was found along the 200-m isobaths. In more than half of all cases, the vertical core profiles of radiocesium concentration generally showed an exponential decreasing trend with depth. However, in the area north of the FDNPP, where the radiocesium concentrations tended to be very low, radiocesium concentrations that had similar or larger magnitude compared with those of the most-surface layer were often found in deeper layers. Relatively good correlations were found between radiocesium concentrations and grain sizes of the most-surface sediment. The vertical profile of radiocesium concentration also had a relationship with grain size. In other case, the radiocesium concentration in the sediment seems to have had a dependence on the radiocesium concentration in bottom seawater, suggesting that the quantity of radiocesium supplied and the grain size were major factors determining the spatial distribution pattern of the radiocesium concentration after the FDNPP accident.

Enormous quantities of radionuclides were released into the ocean via both atmospheric deposition and direct release as a result of the Fukushima Dai-ichi Nuclear Power Plant (FNPP) accident. This study discusses the southward dispersion of FNPP-derived radioactive cesium (Cs) in subsurface waters. The southernmost point where we found the FNPP-derived (134)Cs (1.5-6.8 Bq m(-3)) was 18 °N, 135 °E, in September 2012. The potential density at the subsurface peaks of (134)Cs (100-500 m) and the increased water column inventories of (137)Cs between 0 and 500 m after the winter of 2011-2012 suggested that the main water mass containing FNPP-derived radioactive Cs was the North Pacific Subtropical Mode Water (NPSTMW), formed as a result of winter convection. We estimated the amount of (134)Cs in core waters of the western part of the NPSTMW to be 0.99 PBq (decay-corrected on 11 March 2011). This accounts for 9.0% of the (134)Cs released from the FNPP, with our estimation revealing that a considerable amount of FNPP-derived radioactive Cs has been transported to the subtropical region by the formation and circulation of the mode water.

The Fukushima Dai-ichi Nuclear Power Plant accident in March 2011 released radiocaesium (137Cs and 134Cs) into the North Pacific Ocean. Meridional transects of the vertical distribution of radiocaesium in seawater were measured along 147 °E and 155 °E in October–November 2012, 19 months after the accident. These measurements revealed subsurface peaks in radiocaesium concentrations at locations corresponding to two mode waters, Subtropical Mode Water and Central Mode Water. Mode water is a layer of almost vertically homogeneous water found over a large geographical area. Here we show that repeated formation of mode water during the two winter seasons after the Fukushima accident and subsequent outcropping into surface water transported radiocaesium downward and southward to subtropical regions of the North Pacific. The total amount of Fukushima-derived 134Cs within Subtropical Mode Water, decay-corrected to April 2011, was estimated to be 4.2 ± 1.1 PBq in October–November 2012. This amount of 134Cs corresponds to 22–28% of the total amount of 134Cs released to the Pacific Ocean.

No abstract

The effect of temperature on the growth of Skeletonema ardens, S. costatum sensu stricto, the S. marinoi-dohrnii complex, S. japonicum, S. menzelii, S. pseudocostatum and S. tropicum isolated from Dokai Bay in southern Japan were examined under five to seven different temperatures and an irradiance of 150 mmol m À2 s À1. The effect of irradiance on the growth of the seven Skeletonema species was also examined under a wide range of irradiances ranging from 7-700 mmol m À2 s À1 at 20 C. AllSkeletonema species were able to grow at temperatures ranging from 15 to 25 C. Intra-species differences in specific growth rates of four strains for S. menzelii, and five strains for S. ardens, the S. marinoi-dohrnii complex, S. japonicum and S. tropicum were not significant (Kruskal-Wallis test, P > 0.05). Significant inter-species differences in specific growth rates were observed at 10, 15, 25 and 30 C (Kruskal-Wallis test, P < 0.01; Steel-Dwass test, P < 0.01). The S. marinoi-dohrnii complex and S. japonicum grew faster than other species at the lower temperatures of 10 and 15 C, and S. ardens and S. menzelii grew at the highest temperature of 35 C. The maximum specific growth rates ( max ) from growth-irradiance curves ranged from 1.50 to 3.44 d À1. Threshold values of irradiance (I 0 ) and saturation irradiance (S) for growth ranged from 3.9 to 7.6 mmol m À2 s À1, and from 250 to 740 mmol m À2 s À1, respectively. In Dokai Bay, our results suggested that the occurrence of Skeletonema species should be affected mainly by temperature and less by irradiance. In particular, only two species, the S. marinoi-dohrnii complex and S. japonicum could maintain their populations in the surface water during the cold season, whereas during other periods, all seven species could maintain their population under the strong influence of estuarine circulation, which rapidly flushed the surface water out of Dokai Bay. Temperature and irradiance dependent growth values were in good agreement with their geographical distributions. The S. marinoi-dohrnii complex and S. japonicum were capable of growing in cold regions, but our results suggested that S. ardens and S. menzelii will tend to prefer tropical regions.

The horizontal distribution of radioactive cesium (Cs) derived from the Fukushima Dai-ichi Nuclear Power Plant (FNPP) in the North Pacific is still unclear due to the limitation of direct measurement of the seawater in the open ocean. We present the result of direct observation of radioactive Cs in surface seawater collected from broad area in the western and central North Pacific in July, October 2011 and July 2012. We also conducted a simple particle tracking experiment to estimate the qualitative spatial distribution of radioactive Cs in the North Pacific. ¹³⁴Cs were detected at 94 stations out of 123 stations and ¹³⁷Cs was detected at all stations. The high ¹³⁴Cs and ¹³⁷Cs concentrations more than 10 mBq kg⁻¹ were observed in the area where the northern part of Kuroshio extension at 144° E and 155° E in July 2011, in the area 147° E–175° E around 40° N in October 2011, and the northern part of Kuroshio extension at 155° E and 175° 30´ E in July 2012. Combining the result of direct observations and particle tracking experiment, the radioactive Cs derived from FNPP had been dispersed eastward to the central North Pacific during 2011. It was considered from the horizontal distribution that radioactive Cs was dispersed not only eastward but also north- and southward in the central North Pacific. Pronounced dilution process of radioactive Cs from FNPP during study period is suggested from temporal change in the activity ratio of ¹³⁴Cs/¹³⁷Cs which was decay corrected at 6 April 2011, and relationships between radioactive Cs and temperature

This review summarizes the more than 70 papers published during the 4 years since the Fukushima Dai-ichi nuclear power plant accident that occurred on 11 March 2011, and details the radioactive cesium dispersion pattern in the North Pacific and adjacent seas. The total amount of Fukushima-derived radioactive cesium released into the North Pacific via atmospheric deposition and direct release, spatial and temporal changes in the Pacific coast around the accident site, and the concentration levels of radioactive cesium around the Japanese Islands, not only the Pacific coast but also in adjacent seas, such as Japan Sea, East China Sea are summarized. Based on observational data mostly obtained during 2 years since the accident, and simulation results, oceanic dispersion of radioactive cesium in the entire area of the North Pacific is described. The Fukushima-derived radioactive cesium dispersed eastward as surface water and extended to the eastern side of the North Pacific in 2014, and was also observed via a southward intrusion to subsurface waters as Subtropical Mode Water and Central Mode Water. The radioactive cesium movement related to mode water is important in terms of the circulation of cesium into the ocean interior. Some new technologies and techniques concerning emergency monitoring of radioactivity in the ocean environment are also reported, the effectiveness of which has been demonstrated by use in relation to the Fukushima accident.