Abstract. During the West African summer monsoon season, extended nocturnal stratiform low-level clouds (LLCs) frequently form in the atmospheric boundary layer over southern West Africa and persist long into the following day affecting the regional climate. A unique data set was gathered within the framework of the Dynamics–Aerosol–Chemistry–Cloud Interactions in West Africa (DACCIWA) project, which allows, for the first time, for an observational analysis of the processes and parameters crucial for LLC formation. In this study, in situ and remote sensing measurements from radiosondes, ceilometer, cloud radar and energy balance stations from a measurement site near Savè in Benin are analyzed amongst others for 11 nights. The aim is to study LLC characteristics, the intranight variability of boundary layer conditions and physical processes relevant for LLC formation, as well as to assess the importance of these processes. Based on the dynamic and thermodynamic conditions in the atmospheric boundary layer we distinguish typical nocturnal phases and calculate mean profiles for the individual phases. A stable surface inversion, which forms after sunset, is eroded by differential horizontal cold air advection with the Gulf of Guinea maritime inflow, a cool air mass propagating northwards from the coast in the late afternoon and the evening, and shear-generated turbulence related to a nocturnal low-level jet. The analysis of the contributions to the relative humidity changes before the LLC formation reveals that cooling in the atmospheric boundary layer is crucial to reach saturation, while specific humidity changes play a minor role. We quantify the heat budget terms and find that about 50 % of the cooling prior to LLC formation is caused by horizontal cold air advection, roughly 20 % by radiative flux divergence and about 22 % by sensible heat flux divergence in the presence of a low-level jet. The outcomes of this study contribute to the development of a conceptual model on LLC formation, maintenance and dissolution over southern West Africa.

Aerosol-cloud interactions are central to climate system changes and depend on meteorological conditions. This study identifies distinct thermodynamic regimes and proposes a conceptual framework for interpreting aerosol effects. In the analysis, ten years (2003-2012) of daily satellite-derived aerosol and cloud products are combined with reanalysis data to identify factors controlling Southeast Atlantic stratocumulus microphysics. Considering the seasonal influence of aerosol input from biomass burning, thermodynamic environments that feature contrasting microphysical cloud properties and aerosol-cloud relations are classified. While aerosol impact is stronger in unstable environments, it is mostly confined to situations with low aerosol loading (aerosol index AI ≲ 0.15), implying a saturation of aerosol effects. Situations with high aerosol loading are associated with weaker, seasonally contrasting aerosol-droplet size relationships, likely caused by thermodynamically induced processes and aerosol swelling.

Abstract. The role of aerosols, clouds and their interactions with radiation remain among the largest unknowns in the climate system. Even though the processes involved are complex, aerosol-cloud interactions are often analyzed by means of bivariate relationships. In this study, 15 years (2001)(2002)(2003)(2004)(2005)(2006)(2007)(2008)(2009)(2010)(2011)(2012)(2013)(2014)(2015) of monthly satellite-retrieved near-global aerosol products are combined with reanalysis data of various meteorological parameters to predict satellite-derived marine liquidwater cloud occurrence and properties by means of regionspecific artificial neural networks. The statistical models used are shown to be capable of predicting clouds, especially in regions of high cloud variability. On this monthly scale, lower-tropospheric stability is shown to be the main determinant of cloud fraction and droplet size, especially in stratocumulus regions, while boundary layer height controls the liquid-water amount and thus the optical thickness of clouds. While aerosols show the expected impact on clouds, at this scale they are less relevant than some meteorological factors. Global patterns of the derived sensitivities point to regional characteristics of aerosol and cloud processes.

Abstract. This study presents the first detailed observational analysis of the complete diurnal cycle of stratiform low-level clouds (LLC) and involved atmospheric processes over southern West Africa (SWA). The data used here were collected during the comprehensive DACCIWA (Dynamics-Aerosol-Chemistry-Cloud-Interactions in West Africa) ground-based campaign, which aimed at monitoring LLC characteristics and capturing the wide range of atmospheric conditions related to the West African monsoon flow. In this study, in situ and remote sensing measurements from the supersite near Savè (Benin) collected during a typical day, which is characterized by the onset of a nocturnal low-level jet (NLLJ) and the formation of LLC, are analyzed. The associated dynamic and thermodynamic conditions allow the identification of five different phases related to the LLC diurnal cycle: the stable, jet, stratus I, stratus II, and convective phases. The analysis of relative humidity tendency shows that cooling is a dominant process for LLC formation, which leads to a continuous increase in relative humidity at a maximum rate of 6 % h−1, until finally saturation is reached and LLC form with a cloud-base height near the height of NLLJ maximum. Results of heat budget analysis illustrate that horizontal cold-air advection, related to the maritime inflow, which brings the cool maritime air mass and a prominent NLLJ wind profile, has the dominant role in the observed strong cooling of −1.2 K h−1 during the jet phase. The contribution from horizontal cold advection is quantified to be up to 68 %, while radiative cooling and sensible heat flux divergence both contribute 16 % to the observed heat budget below the NLLJ maximum. After the LLC form (stratus phases I and II), turbulent mixing is an important factor leading to the cooling below the cloud base, while strong radiative cooling at the cloud top helps to maintain thick stratus.

<p><strong>Abstract.</strong> During the West African summer Monsoon season, extended nocturnal stratiform low-level clouds (LLC) frequently form in the atmospheric boundary layer over southern West Africa and persist long into the following day affecting the regional climate. A unique data set was gathered within the framework of the Dynamics-Aerosol-Chemistry-Cloud-Interactions in West Africa (DACCIWA) project, which allows, for the first time, for an observational analysis of the processes and parameters decisive for LLC formation. In this study, in situ and remote sensing measurements from radiosondes, ceilometer, cloud radar and energy balance stations from a measurement site near Savè in Benin are analyzed amongst others for 11 nights. The aim is to study LLC characteristics, the intra-night variability of boundary layer conditions and physical processes relevant for LLC formation, as well as to assess the importance of these processes. Typical nocturnal phases are identified and mean profiles are calculated for the individual phases revealing pronounced differences: a stable surface inversion, which forms after sunset, is eroded by differential horizontal cold air advection with the Gulf of Guinea maritime inflow, a cool air mass propagating northwards from the coast in the late afternoon and the evening, and shear-generated turbulence related to a nocturnal low-level jet. The analysis of the contributions to the relative humidity changes before the LLC formation reveals that cooling in the atmospheric boundary layer is decisive to reach saturation, while moisture changes play a minor role. We quantify the heat budget terms and find that about 50 % of the cooling prior to the LLC formation is caused by horizontal cold air advection, roughly 20 % by radiative flux divergence and about 22 % by sensible heat flux divergence in the presence of a low-level jet. The outcomes of this study contribute to the development of a conceptual model on LLC formation, maintenance and dissolution over southern West Africa.</p>