Textile-based stretchable electronic devices are one of the best candidates for future wearable applications, as they can simultaneously provide high compliance and wearing comfort to the human body. Stretchable conductive textile is the fundamental building block for constructing high-performance textile-based stretchable electronic devices. Here, we report a simple strategy for the fabrication of stretchable conductive fabric using commercial knitted cloth as a substrate. Briefly, we coated the fibers of the fabric with a thin layer of poly(styrene-block-butadiene-block-styrene) (SBS) by dip-coating. Then, silver nanoparticles (AgNPs) were loaded on the fabric by sequential absorption and in situ reduction. After loading AgNPs, the conductivity of the fabric could be as high as ∼800 S/m, while its maximal strain at break was higher than 540%. Meanwhile, such fabric also possesses excellent permeability, robust endurance to repeated stretching, long-time washing, and mechanical rubbing or tearing. We further approve that the fabric is less cytotoxic to mammalian skin and antibacterial to microbial, making it safe for on-skin applications. With these multifarious advantages, the fabric developed here is promising for on-skin wearable applications. As a proof-of-concept, we demonstrate its use as an electrode for collecting electrocardiograph signals and electrothermal therapy.

Elastic fiber conductors are advantageous for applications in wearable electronics due to their small size, light weight, and excellent integration ability. Here, we report the fabrication of elastic fiber conductors with a three-dimensional (3D) porous structure using electrospun thermoplastic elastomer (TPE) microfibers and silver nanoparticles (AgNPs) as the building blocks. With the 3D porous structure, such a fiber is highly permeable to gases and liquids. As such, the performance of the fiber in many applications of wearable electronics (especially wearable sensors and detectors) can be improved significantly. Benefitting from the excellent processability of TPE and dispersibility of AgNPs, the fiber is highly compatible with thermal and solvent welding. In addition, the fiber also possesses super stretchability, high conductivity, and robust endurance to deformation. As a proof-of-concept application, we demonstrate that a ropeshaped capacitor made by plying one pair of such fibers can detect the volume change of artificial sweat with 17-times higher sensitivity than the capacitor using nonporous fibers as electrodes. We further demonstrate that, by integrating two groups of perpendicularly arranged fibers into a monolithic porous mat, sensitive matrix-addressed monitoring of artificial sweat can be realized.

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