We report direct printing and photo-thermal reduction of graphite oxide (GO) to obtain a highly porous pattern of interdigitated electrodes, leading to a supercapacitor on a flexible substrate. Key parameters optimized include the amount of GO delivered, the suitable photo-thermal energy level for effective flash reduction, and the substrate properties for appropriate adhesion after reduction. Tests with supercapacitors based on the printed-reduced GO showed performance comparable with commercial supercapacitors: the energy densities were 1.06 and 0.87 mWh/cm3 in ionic and organic electrolytes, respectively. The versatility in the architecture and choice of substrate makes this material promising for smart power applications.
Herein, the color gamut change by optical crosstalk between sub-pixels in high-resolution full-color organic light-emitting diode (OLED) microdisplays was numerically investigated. The color gamut of the OLED microdisplay decreased dramatically as the pixel density of the panel increased from 100 pixels per inch (PPI) to 3000 PPI. In addition, the increase in thickness of the passivation layer between the bottom electrode and the top color filter results in a decrease in the color gamut. We also calculated the color gamut change depending on the pixel structures in the practical OLED microdisplay panel, which had an aspect ratio of 32:9 and a pixel density of 2,490 PPI. The fence angle and height, refractive index of the passivation layer, black matrix width, and white OLED device structure affect the color gamut of the OLED microdisplay panel because of the optical crosstalk effect.
We improved biometric authentication security using dual recognition based on fingerprint image detection and skin-temperature-change sensing under quantum dot light-emitting diode (QLED) displays. QLEDs are more advantageous than organic light-emitting diodes (OLEDs) in terms of the contrast classification of patterns such as those in fingerprint recognition, owing to their narrow full-width-half-maximum. In this work, scattered, transmitted, and reflected light was captured from the top of the QLED, improving the digital luminance by 25%, as compared with that of OLEDs, because the electroluminescence spectra of the QLED were sustained, whereas those of the OLED were distorted by the generated noise peaks. A QLED with eight apertures sized up to tens of micrometers, mimicking the actual wiring structure of commercialized smartphones, was implemented to detect human fingerprints. The QLED using reduced graphene oxide as the temperature sensor detected temperature changes instantaneously upon finger touch, showing a 2% temperature response based on the human body temperature; however, the temperature change was less than 0.1% for spoof fingerprints printed on paper. Thus, this study successfully enhanced biometric authentication security, through fingerprint recognition based on image sensing using an optical system with micrometer-sized apertures and skin-temperature detection under QLED displays.
We present an adherable temperature sensor on aramid fiber filament coated with reduced graphene oxide (rGO) and poly(diallyldimethylammonium chloride) (PDADMAC) complex. The PDADMAC dispersed in a graphene oxide aqueous solution was dried and reduced to an rGO-PDADMAC complex with laser irradiation. The rGO-PDADMAC sensor was characterized with a scanning electron microscope and Raman spectroscopy. The rGO-PDADMAC sensor showed a negative temperature coefficient resistance change at 40% relative humidity (RH). Furthermore, the sensor successfully detected 58% resistance variation from 25°C to 100°C as the pristine rGO sensor showed 61% resistance variation on a rigid surface. Also, the rGO-PDADMAC sensor demonstrated long-term reliability of 3% sensitivity for 7 days in normal room conditions at 25°C and 40% RH. Additionally, the adherable temperature sensor of the rGO-PDADMAC complex viscous to the porous structure of aramid fiber detected 55% sensitivity from 25°C to 100°C.
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