Magnetic ordering can tune optical properties of photoluminescent dilute magnetic semiconductors. The results of a magnetic field dependent photoluminescence ͑PL͒ up to 50 T above and below ferromagnetic transition temperature T C in Mn-doped ZnS nanocrystals have been reported here. The PL intensity corresponding to internal transition between states of Mn significantly decreases with application of magnetic field below T C but no such suppression was observed above T C even at 50 T. The zero-field PL intensity also exhibits continuous suppression with decreasing temperature in the ferromagnetic state. The PL intensity profiles could be fitted consistently using a model of magnetic-ordering-induced spin-sensitive energy transfer to Mn states below T C .
The spin coherence of photoexcited electrons in ZnSe∕BeTe type-II quantum wells has been investigated by the time-resolved Kerr rotation technique. Fast and efficient escape of photoexcited holes from the ZnSe layers to the BeTe layers suppresses the electron-hole recombination and their exchange interaction. This effect leads to the formation of dense electrons in ZnSe layers and long electron spin dephasing time reaching a value of 6.1ns at 1.4K.
Photoluminescence (PL) spectra occurred as a spatially direct optical transition inside of the ZnSe layer in undoped ZnSe∕BeTe∕ZnSe type-II quantum structures have been studied. We have found that the charged exciton transition was observed at the lower energy side of the exciton transition in the spatially direct PL. The formation of the charged exciton was attributed to the accumulated electrons in the ZnSe layer after the photoexcitation accompanied by the holes being escaped from this well and injected into the BeTe layer.
We investigate the electron-phonon coupling in CH 3 NH 3 PbX 3 lead halide perovskites through the observation of Landau levels and high-order excitons at weak magnetic fields, where the cyclotron energy is significantly smaller than the longitudinal optical phonon energy. The reduced masses of the carriers and the exciton binding energies obtained from these data are clearly influenced by polaron formation. We analyze the field-dependent polaronic and excitonic properties, and show that they can be quantitatively reproduced by the Fröhlich large polaron model.
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