We have performed muon spin relaxation measurements of the frustrated kagome lattice spin system SrCr8Ga4019. Our results demonstrate the slowing down of the Cr spin fluctuations when cooling toward the susceptibility-cusp temperature Tg 3 5 K The saturation of the relaxation rate below Tg, together with its weak dependence on longitudinal field (LF) between 0 and 2 kG, indicates the presence of dynamic spin fluctuations persisting even at T -100 mK without static order parameter. We propose a spin-liquid type ground state to explain an undecouplable Gaussian shape of the relaxation function observed at T~T , .
The magnetic susceptibility, high field magnetization, and specific heat measurements of Cu3(CO3)2(OH)2, which is a model substance for the frustrating diamond spin chain model, have been performed using single crystals. Two broad peaks are observed at around 20 and 5 K in both magnetic susceptibility and specific heat results. The magnetization curve has a clear plateau at one third of the saturation magnetization. The experimental results are examined in terms of theoretical expectations based on exact diagonalization and density matrix renormalization group methods. An origin of magnetic anisotropy is also discussed.
We have measured magnetic susceptibility and 51V NMR of CaV2O4, a model substance for a frustrated S = 1 spin chain with competing first- and second-neighbor anti-ferromagnetic interactions. Both the low-temperature magnetic susceptibility and the NMR Knight shift did not go down to zero as the temperature was lowered, suggesting that a spin gap is not present in CaV2O4. The absence of a spin gap gives us a clear contrast to the case of the nonfrustrated spin chains, which should have the Haldane gap. Recently published theoretical results for S = 1 XY or XXZ spin chain indicate that the gapless chiral phase could appear in a relatively broad region. Experimental results are discussed in terms of these theoretical predictions. A spin-freezing anomaly was observed at 20 K, reflecting the spin-frustrating nature of the system. PACS Nos.: 75.30, 75.50
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