We have measured absolute triple differential cross sections for photo-double ionization of helium at 20 eV excess. The measurement covers the full ranges of energy sharing and emission angles of the two photoelectrons. We compare our data for selected geometries with the convergent close-coupling (CCC) calculations as well as 2SC calculations by Pont and Shakeshaft and 3C calculations by Maulbetsch and Briggs. In terms of the absolute magnitude and the trend in the shapes of the triple differential cross section for different geometries we find good agreement of the CCC and published 2SC calculations with our measurement, though differences with respect to the observed shape of individual patterns still exist.
We measure fully differential cross sections for photo-double-ionization of helium at energies 1, 6, and 20 eV above threshold. The data have been obtained by measuring in coincidence the momentum vector of the He 2ϩ ion and one of the electrons. Using time-of-flight and imaging techniques, we cover a solid angle of 25-100 % 4 of the final-state continuum of all particles. Therefore the experiment is not confined to any particular set of angles or energy sharing, and allows for a reliable absolute calibration. We present momentum distributions of the ions and a comprehensive set of differential cross sections for electron emission. The latter are on an absolute scale and cover both equal and unequal energy sharing-for both the fast and the slow electron fixed-and a wide range of polar angles. We also present the first data for noncoplanar geometry. For all energies the cross section is sharply peaked around the coplanar emission, i.e., both electrons are preferentially emitted in the plane of the recoiling ion and the photon polarization direction. For most of the geometries the shape of the cross sections is well described by fourth-order Wannier theory calculations.
We have used COLTRIMS to measure the angular distribution of electrons released from the K-shell of N 2 and the carbon K-shell of CO by absorption of one linear polarized photon. For each ionization event which leads to two charged fragments we determine the angle of the photoelectron with respect to the fragment ion momenta. In addition we determine the charge state and energy of the molecular fragments. We find a breakdown of the axial recoil approximation for CO for kinetic energy releases below 10.2 eV, whereas for N 2 that approximation is found to be valid for all fragment energies. Furthermore, the photoelectron emission spectrum for N 2 is found to be the same for the molecular breakup channels producing N + N + and N + N ++ .
On page 1026, the last sentence of the second paragraph should read, "However, Lablanquie et al.[5] could show from their ͑g, 2e͒ data that at E exc 4 eV the ratio K 0 (which is proportional to the a u term in their notation) to K 1 is small, typically down to 1͞19."
We report the observation of an interference between the electric dipole (E1) and the magnetic quadrupole (M2) amplitudes for the linear polarization of the Ly-α1 (2p3/2→1s1/2) radiation of hydrogenlike uranium. This multipole mixing arises from the coupling of the ion to different multipole components of the radiation field. Our observation indicates a significant depolarization of the Ly-α1 radiation due to the E1-M2 amplitude mixing. It proves that a combined measurement of the linear polarization and of the angular distribution enables a very precise determination of the ratio of the E1 and the M2 transition amplitudes and the corresponding transition rates without any assumptions concerning the population mechanism for the 2p3/2 state.
The four-body breakup of spatially aligned D 2 by 58.8 eV photons from the Advanced Light Source has been investigated by measuring the three dimensional momentum vectors of both fragment ions and one of the two electrons in coincidence. Energy and angular correlation between ions and electrons is discussed. We find rotational symmetry of the electron angular distribution around the polarization vector of the light and significant differences between helium and D 2 as well as between molecular alignment parallel and perpendicular to the polarization axis. [S0031-9007(98)
Using 98% linearly polarized radiation at the European Synchrotron Radiation Facility in Grenoble, the performance of a prototype two-dimensional microstrip Ge(i) detector for x-ray imaging and as a Compton polarimeter has been evaluated. Using the energy and position sensitivity of the detector, the ability to obtain a complete reconstruction of the Compton event has been demonstrated. The modulation coefficient of the polarimeter is in good agreement with the theoretical limit of a perfect detector.
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