SUMMARYCollisions between vapour-grown ice crystals and a riming target, representing a graupel pellet falling in a thunderstorm, were shown by Reynolds, Brook and Gourley to transfer substantial charge, which they showed to be adequate to account for the development of charge centres leading to lightning in thunderstorms. Related experiments by Takahashi and Jayaratne et al. determined that the sign of charge transferred is dependent on the cloud liquid water content and on cloud temperature. There are marked differences between the results of Takahashi and Jayaratne in the details of the dependence they noted of the sign of graupel charging on cloud water and temperature. More recently, Pereyra et al. have shown that results somewhat similar in form to those of Takahashi are obtained by modifying the experimental technique used to prepare the clouds of ice crystals and supercooled water droplets used in the experiments.In order to help resolve the reason for the differences in charge transfer results in various studies, work has continued in the Manchester laboratory with a modified cloud chamber in which the cloud conditions of the crystals and droplets may be controlled independently. Results indicate a profound effect on the charge sign of the particle growth conditions in the two clouds involved. For example, by suitable adjustments to the water contents of the two clouds, graupel is charged negatively by rebounding ice crystal collisions at higher cloud water contents than have been noted previously. It is suggested that the most important influence on charge sign is the relative diffusional growth rate of the two ice surfaces at the moment of impact and that this is affected by an increase in cloud supersaturation experienced by the ice crystals during the cloud mixing process just prior to collision. A range of cloud conditions is used in the present work in order to help determine the reasons for the various results reported previously.Examination of some thunderstorm observations in the context of the present results points to the importance of mixing on the sign of the charge transferred during particle collisions when two cloud regions of different histories mix together.
SUMMARYLaboratory studies of a thunderstorm charging mechanism involving rebounding collisions between ice crystals and riming graupel pellets, have shown the importance of the growth conditions of the interacting ice particles on the sign of the charge transferred. The present study shows a new result: if an ice crystal is not in thermal equilibrium with the environment (immediately following the mixing of two clouds at different saturations) the crystal surface may experience an enhanced growth rate that can influence the sign of the charge transfer and promote negative rimer charging. Furthermore, when an ice crystal in ice saturation conditions is introduced to a cloud at water saturation, leading to transient growth and heating, the period of thermal nonequilibrium is shown to be sufficiently brief that the enhanced negative rimer charging is short lived. These results suggest that the earlier conclusions of Berdeklis and List-that the cloud saturation conditions around a growing ice crystal impart to the crystal surface a property that is carried with it and that influences the sign of subsequent charge transfer-are unfounded. The discrepancy is because in their laboratory simulations of thunderstorm conditions there is adequate time for the growing ice crystal surface to come to equilibrium with its environment. The established concept of the relative diffusional growth rate of the interacting surfaces controlling the sign of charge transfer, such that the faster growing surface charges positively, is consistent with the observations.
[1] Laboratory measurements of the sign of electric charge transfer separated in rebounding collisions between large ice crystals and a graupel pellet growing by riming are analyzed. In these experiments, the usual negative rimer charging regime noted at temperatures below about À10°C at moderate liquid water contents is reversed to positive when the crystals have grown larger. The experiments were performed with an impact velocity of 5.5 m s À1 , the ambient temperature was varied in the range À15 to À26°C with an effective water content from 0.5 to 3 g m À3 . A cloud particle imager shows a clear correlation between the rimer charge sign reversal to positive and the presence of a high proportion of irregular and large ice crystals or aggregates in the cloud. The results suggest that in collisions between graupel and these ice particles the graupel will charge positively while the irregular particles carry away a negative charge. These are the first measurements of this kind of collision and the findings may have important implications in the thunderstorm electrification process. Citation: Avila,
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