Recently there have been major increases in water colour and dissolved organic carbon (DOC) in many forest lakes that serve as drinking water reservoirs in the southern part of Norway. We studied changes in the physical and chemical properties in (I) a selected group of lakes and (II) raw water from the municipal waterworks of Oslo since 1983 and 1976, respectively. The largest increase in DOC and water colour occurred between 1997 and 2001. Statistically significant correlations are seen between water colour and accumulated amounts of precipitation, while variation in temperature had no apparent Aquatic Sciences effect. Despite significant reduction in sulphate concentrations in precipitation and lake waters since 1980, the lakes were more acidic in 2000 and 2001 than in previous years. Increases in colour and acidity, together with somewhat minor changes in DOC concentrations, indicate changes in the physical and chemical properties of the natural organic matter (NOM). Alteration in properties of NOM is most probably caused by increased precipitation that has changed the water pathways in the catchments and increased the leaching of organic components from the upper forest floor.

Recent reports of increasing iron (Fe) concentrations in freshwaters are of concern, given the fundamental role of Fe in biogeochemical processes. Still, little is known about the frequency and geographical distribution of Fe trends or about the underlying drivers. We analyzed temporal trends of Fe concentrations across 340 water bodies distributed over 10 countries in northern Europe and North America in order to gain a clearer understanding of where, to what extent, and why Fe concentrations are on the rise. We found that Fe concentrations have significantly increased in 28% of sites, and decreased in 4%, with most positive trends located in northern Europe. Regions with rising Fe concentrations tend to coincide with those with organic carbon (OC) increases. Fe and OC increases may not be directly mechanistically linked, but may nevertheless be responding to common regional‐scale drivers such as declining sulfur deposition or hydrological changes. A role of hydrological factors was supported by covarying trends in Fe and dissolved silica, as these elements tend to stem from similar soil depths. A positive relationship between Fe increases and conifer cover suggests that changing land use and expanded forestry could have contributed to enhanced Fe export, although increases were also observed in nonforested areas. We conclude that the phenomenon of increasing Fe concentrations is widespread, especially in northern Europe, with potentially significant implications for wider ecosystem biogeochemistry, and for the current browning of freshwaters.

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Long-term monitoring of surface water quality has shown increasing concentrations of colored dissolved organic matter (CDOM) across large parts of the northern latitudes. This has increased purification costs for domestic water works. Appropriate abatement actions require better knowledge of the governing factors for the increase, and this has motivated a growing scientific interest in understanding the factors and mechanisms promoting the CDOM increase. A proposed water color model for an important raw water source for Oslo, Norway, is based on the precipitation's amount and mobile ion concentration. The model explained more than 93% of the temporal variation in CDOM between 1983 and 2008. The model structure was also tested on three adjacent raw water sources and was found to explain 75-82% of the CDOM development throughout the same period. The long-term trend of increasing CDOM was closely related to the decline in sulfate and chloride concentrations in precipitation. Furthermore, interannual fluctuations in CDOM were explained by variation in predominant water flow paths, depending on amounts and intensity of precipitation, both of which are predicted to increase in several parts of the northern latitudes according to climate change scenarios.