-Sr and Nd isotope ratios, together with lithophile trace elements, have been measured in a representative set of igneous rocks and Lewisian gneisses from the Isle of Rum in order to unravel the petrogenesis of the felsic rocks that erupted in the early stages of Palaeogene magmatism in the North Atlantic Igneous Province (NAIP). The Rum rhyodacites appear to be the products of large amounts of melting of Lewisian amphibolite gneiss. The Sr and Nd isotopic composition of the magmas can be explained without invoking an additional granulitic crustal component. Concentrations of the trace element Cs in the rhyodacites strongly suggests that the gneiss parent rock had experienced Cs and Rb loss prior to Palaeogene times, possibly during a Caledonian event. This depletion caused heterogeneity with respect to 87 Sr/ 86 Sr in the crustal source of silicic melts. Other igneous rock types on Rum (dacites, early gabbros) are mixtures of crustal melts and and primary mantle melts. Forward Rare Earth Element modelling shows that late stage picritic melts on Rum are close analogues for the parent melts of the Rum Layered Suite, and for the mantle melts that caused crustal anatexis of the Lewisian gneiss. These primary mantle melts have close affinities to Mid-Oceanic Ridge Basalts (MORB), whose trace element content varies from slightly depleted to slightly enriched. Crustal anatexis is a common process in the rift-to-drift evolution during continental break-up and the formation of Volcanic Rifted Margins systems. The 'early felsic-later mafic' volcanic rock associations from Rum are compared to similar associations recovered from the now-drowned seaward-dipping wedges on the shelf of SE Greenland and on the Vøring Plateau (Norwegian Sea). These three regions show geochemical differences that result from variations in the regional crustal composition and the depth at which crustal anatexis took place.

The Southern Mountains Zone of the Rum Central Complex lies inside a major ring fault and comprises an intricate association of country-rock outcrops, breccias and rhyodacite. The breccias and rhyodacite were long thought to be products of subterranean explosion and intrusion, respectively. Here, we report new observations that support re-interpretation of these units as mass movement deposits and ignimbrites. The most abundant breccias (Coire Dubh-type) consist mainly of countryrock clasts < 1 m in diameter in a sand or silt matrix. Internally bedded and graded, and interlayered with sandstones and lithic tuffs, these breccias are interpreted as debris flow and stream flow deposits. Rhyodacite sheets show gradational or sharp, concordant contacts with Coire Dubh-type breccias, and display graded basal lithic tuffs and graded fiamme swarms. These sheets are interpreted as moderately to densely welded rhyodacite ignimbrites (25-100 m thick). A steep body of fragmented (fiammebearing) rhyodacite with intrusive non-fragmented contacts is interpreted as an ignimbrite vent system. The rhyodacite and breccia succession is over 200 m thick and unconformably overlies a structurally uplifted Precambrian basement, within which there is also evidence of later subsidence. Outcrops of potential caldera-collapse 'megabreccia' are more structurally consistent than previously thought, and are re-interpreted here as coherent segments of Precambrian country rock (caldera floor). The Southern Mountains Zone breccias and rhyodacites respectively reflect sedimentary and pyroclastic processes acting in response to a complex tectonic interplay of intrusion-related uplift and caldera subsidence.

We present U–Pb (LA-ICP-MS) data on detrital zircon from the Late Precambrian terrigenous rocks of the Baikal Group and Ushakovka Formation, western Cisbaikalia (southern flank of the Siberian craton). The sources of clastic material for the studied sediments are interpreted. The youngest group of detrital zircon grains from the upper Baikal Group and Ushakovka Formation permits assigning these sediments to the Vendian. The lack of Mesoproterozoic detrital zircon in most of the analyzed samples confirms the hypothesis of a global (~1 Gyr) break in endogenic activity within the southern flank of the Siberian craton through the Precambrian. The abundance of Neoproterozoic zircon in sandstones from the upper horizons of the Baikal Group and the Ushakovka Formation might be due to the shrinkage of the ocean basin as a result of the convergence of the craton with the microcontinents and island arcs within the Paleoasian ocean.

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The Rum Igneous Centre comprises two early marginal felsic complexes (the Northern Marginal Zone and the Southern Mountains Zone), along with the later central ultrabasic–basic layered intrusions. These marginal complexes represent the remnants of near-surface to eruptive felsic magmatism associated with caldera collapse, examples of which are rare in the North Atlantic Igneous Province. Rock units include intra-caldera collapse breccias, rhyolitic ignimbrite deposits and shallow-level felsic intrusions, as well the enigmatic ‘Am Màm intrusion breccia’. The latter comprises a dacitic matrix enclosing lobate basaltic inclusions (~1–15 cm) and a variety of clasts, ranging from millimetres to tens of metres in diameter. These clasts comprise Lewisian gneiss, Torridonian sandstone and coarse gabbro. Detailed re-mapping of the Am Màm intrusion breccia has shown its timing of emplacement as syn-caldera, rather than pre-caldera as previously thought. Textural analysis of entrained clasts and adjacent, uplifted country rocks has revealed their thermal metamorphism by early mafic intrusions at greater depth than their present structural position. These findings provide a window into the evolution of the early mafic magmas responsible for driving felsic magmatism on Rum. Our data help constrain some of the physical parameters of this early magma–crust interaction and place it within the geochemical evolution of the Rum Centre.

Large-volume pyroclastic eruptions are not known from the basalt-dominated British Palaeogene Igneous Province (BPIP), although silicic magmatism is documented from intra-caldera successions in central volcanoes and from small-volume ash-layers in the associated lava fields. Exceptions are the Sgùrr of Eigg (58.7 Ma) and Òigh-sgeir pitchstones in the Inner Hebrides (>30 km apart), which have been conjectured to represent remnants of a single large silicic event. Currently available major element data from these outcrops differ, however, creating a need to test if the two pitchstones are really related. We employ a systematic array of methods ranging from mineralogy to isotope geochemistry and find that samples from the two outcrops display identical mineral textures and compositions, major- and trace elements, and Sr-Nd-Pb-O isotope ratios, supporting that the two outcrops represent a single, formerly extensive, pyroclastic deposit. Available isotope constraints suggest a vent in the Hebridean Terrane and available radiometric ages point to Skye, ~40 km to the North. A reconstructed eruption volume of ≥5km3 DRE is derived, suggesting a VEI 5 event or larger. We therefore argue, contrary to long-held perception, that large-volume silicic volcanism and its associated climatic effects were likely integral to the BPIP during the opening of the North Atlantic.

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