The probable site of extraction and production of Pompeian‐style leucite‐bearing millstones, singled out by Peacock (1980, 1986) in the vicinity of Orvieto, and the outcropping of the ‘Leucitophyre’ lava have been systematically studied employing standard petrographic and geochemical methods (optical microscopy and ICP–AES/MS spectrometry). The combination of petrochemical data, previously very poor, allowed us definitively to exclude the possible ‘overlap’ of phonolitic and tephri‐phonolitic lavas from other Quaternary Volcanic Districts of Latium, and provides a helpful tool for future work on leucitite millstones. Consequently, the databank obtained has been used to attribute the origin of five Roman millstones discovered in three archaeological sites in central Italy (Latium and Marche). It has also been useful to verify the geological provenance of some Sicilian and French leucitite millstones analysed by previous workers. The results point to a provenance from the Orvieto area, with the exception of the millstones from Sicily, for which a different origin was hypothesized.
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