We report resistivity measurements performed on KFe 2 As 2 single crystals down to T = 0.3 K and in magnetic fields up to 17.5 T. The in-plane resistivity vs. T curve has a convex shape down to ∼50 K and shows a T 2 dependence below ∼45 K. The ratio of the c-axis to in-plane resistivities is ∼10 at room temperature and ∼40 at 4.2 K. The superconducting
Fe-Kβ X-ray emission spectroscopy measurements reveal an asymmetric doping dependence of the magnetic moments μ
bare in electron- and hole-doped BaFe2As2. At low temperature, μ
bare is nearly constant in hole-doped samples, whereas it decreases upon electron doping. Increasing temperature substantially enhances μ
bare in the hole-doped region, which is naturally explained by the theoretically predicted crossover into a spin-frozen state. Our measurements demonstrate the importance of Hund’s-coupling and electronic correlations, especially for hole-doped BaFe2As2, and the inadequacy of a fully localized or fully itinerant description of the 122 family of Fe pnictides.
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