Based on direct numerical simulations of the coupled motion of particles and fluid, this study analyzes the collective hydrodynamic and colloidal effects of flowing microparticles during the formation of different 3D clogging patterns at a pore entrance. Simulations of flowing suspensions through a pore with various simulation conditions show that particle concentration and surface interactions play a major role in the occurrence of the bridging phenomenon (simultaneous adhesion of many particles). In the absence of DLVO repulsive forces, plugging is characterized by the temporal reduction of the bulk permeability when increasing the volume fraction of the flowing suspension up to 20%. Under these conditions, different structures of particle aggregates (from cluster to cake plug) are formed at the pore entrance yielding different evolution rates of hydrodynamic resistance to the flow. Taking into account DLVO repulsive forces in simulations for a particle concentration equal to 10%, we observe the transition from dendritic structures (for low repulsion) to dense aggregates (for high repulsion). At high DLVO repulsive forces, the scenario of pore clogging is controlled by the collective behavior of many interacting particles. It leads to the formation of a jamming phase (Wigner glass phase) with transient clusters of interacting particles at the pore entrance. The network of jammed particles collapses when the force chains among the particles are overcome by the flow stress. The build-up and the collapse of the jammed phase at the pore entrance induce temporal permeability fluctuations. According to the relative magnitude of particle-particle and particle-wall interactions, when the jammed phase is disorganized by the flow, the residual force in the network can accelerate particles and lead to particle adhesion at the wall inducing a pore blockage and a rapid reduction of the bulk permeability.
OATAO is an open access repository that collects the work of Toulouse researchers and makes it freely available over the web where possible. This is an author-deposited version published in : http://oatao.univ-toulouse.fr/ Eprints ID : 6835 b s t r a c tPrediction of pore fouling by microparticles is still challenging and remains a difficult step to optimize membrane and filtration processes. The scientific issue consists in determining the relevant operation parameters controlling the capture of particles and the clogging of the filter. In this study, we have developed for a dead-end and cross-flow filtration a poly-dimethylsiloxane (PDMS) device which allows direct observation of the clogging dynamics of microchannels (20 lm wide) by micrometric particles (5 lm diameter). The experiments highlight the formation of different 3D clogging patterns according to the filtration conditions (particle concentration, flowrate, particle flux density and physical-chemical conditions of suspension). Besides, we have determined under which specific conditions of filtration, the latex microparticles are captured and form arches, clusters or dendrites. For each type of structure, the temporal dynamics of the particle deposition are analyzed by means of the average thickness of deposit. The critical conditions for the formation of arches leading to deposit formation have been identified in term of a combination of operating conditions: the particle concentration and the particle velocity. A critical particle flux density yielding pore clogging is then observed and characterized. Studying these experimental results helps to identify pore clogging mechanisms: deposition, interception and bridging.
a b s t r a c tThe dynamic formation of 3D structures of microparticle aggregates blocking the flow through straight microchannels is investigated by direct numerical simulation of the coupled motion of particles and fluid. We use the Force Coupling Method to handle simultaneously multibody hydrodynamic interactions of confined flowing suspension together with particle-particle and particle-wall surface interactions leading to adhesion and aggregation of particles. The basic idea of the Force Coupling Method relies on a multipole expansion of forcing terms (added to the Navier-Stokes equations) accounting for the velocity perturbation induced by the presence of particles in the fluid flow. When a particle reaches the wall or an attached particle, we consider that the adhesion is irreversible and this particle remains fixed. We investigate the kinetics of the microchannel blockage for several solid volumetric concentrations and different surface interaction forces. Many physical quantities such as the temporal evolution of the bulk permeability, capture efficiency, modification of the fluid flow and forces acting on attached particles are analyzed. We show that physical-chemical interactions, modeled by DLVO forces, are essential features which control the blockage dynamics and aggregate structure. IntroductionThe physics of transport, deposition, detachment and reentrainment of colloidal particles suspended in a fluid are of major interest in many areas of fluids engineering: fouling of heat exchangers, contamination of nuclear reactors, plugging of filtration membranes and occlusion of human veins, deposits in microelectronics and in the paper industry. In many solid/liquid separation processes such as micro-filtration or ultrafiltration of water, the limitation of the process performance is related to the fouling of filtration devices. To prevent or control the occurrence of fouling, it is necessary to achieve a better understanding of the respective roles of physical-chemical phenomena and hydrodynamic interactions in a confined suspension of particles. Non-hydrodynamic surface interactions and the adhesion of particles onto solid surfaces are the essential features to be modeled. However, mainly because of a complex interplay between the hydrodynamics of the flow, the physical-chemical properties of the filtered suspensions (often in a colloidal state) and the nature of the solid material, predicting fouling dynamics is still challenging.Different experimental techniques and numerical approaches have been developed to achieve new insights on the local structure of particle aggregates and the kinetics of blockage. Sharp and Adrian [4], by means of experiments in microtubes, observed blockage due to arch formation. The experiments were performed using liquids seeded with polystyrene beads at low volumetric concentration. They showed that a stable balance between the hydrodynamic forces and contact forces (mainly solid friction) between particles and the wall provokes the formation of arches. Wyss et al.[5] stu...
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