A novel theoretical approach to the dynamics analysis of excitation and dephasing of plasmon modes in nanoparticles is presented. This approach is based on the biorthogonal plasmon mode expansion, and it leads to the predictions of time dynamics of excitation of specific plasmon modes as well as their steady state amplitude and their decay. Temporal characteristics of plasmon modes in nanoparticles are expressed in terms of their shapes, permittivity dispersion relations, and excitation conditions. In the case of the Drude model, analytical expressions for time-dynamics of plasmon modes are obtained.
In the present Letter, we demonstrate how the design of metallic nanoparticle arrays with large electric field enhancement can be performed using the basic paradigm of engineering, namely the optimization of a well-defined objective function. Such optimization is carried out by coupling a genetic algorithm with the analytical multiparticle Mie theory. General design criteria for best enhancement of electric fields are obtained, unveiling the fundamental interplay between the near-field plasmonic and radiative photonic coupling. Our optimization approach is experimentally validated by surface-enhanced Raman scattering measurements, which demonstrate how genetically optimized arrays, fabricated using electron beam lithography, lead to order of ten improvement of Raman enhancement over nanoparticle dimer antennas, and order of one hundred improvement over optimal nanoparticle gratings. A rigorous design of nanoparticle arrays with optimal field enhancement is essential to the engineering of numerous nanoscale optical devices such as plasmon-enhanced biosensors, photodetectors, light sources and more efficient nonlinear optical elements for on chip integration.
A transmission line (TL) model describing the propagation of electric signals along metallic single wall carbon nanotube (CNT) interconnects is derived in a simple and self-consistent way within the framework of the classical electrodynamics. The conduction electrons of metallic CNTs are modelled as an infinitesimally thin cylindrical layer of a compressible charged fluid with friction, moving in a uniform neutralizing background. The dynamic of the electron fluid is studied by means of the linearized hydrodynamic equations with the pressure assumed to be that of a degenerate spin- 12 ideal Fermi gas. Transport effects due to the electron inertia, quantum fluid pressure and electron scattering with the ion lattice significantly influence the propagation features of the TL. The simplicity and robustness of the fluid model make the derivation of the TL equations more straightforward than other derivations recently proposed in the literature and provide simple and clear definitions of the per unit length (p.u.l.) TL parameters. In particular, this approach has provided a new circuit model that can be used effectively in the analysis of networks composed of CNT transmission lines and lumped elements. The differences and similarities between the proposed model and those given in the literature are highlighted
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