We discovered that chiral nanoneedles fabricated by vortex laser ablation can be used to visualize the helicity of an optical vortex. The orbital angular momentum of light determines the chirality of the nanoneedles, since it is transferred from the optical vortex to the metal. Only the spin angular momentum of the optical vortex can reinforce the helical structure of the created chiral nanoneedles. We also found that optical vortices with the same total angular momentum (defined as the sum of the orbital and spin angular momenta) are degenerate, and they generate nanoneedles with the same chirality and spiral frequency. DOI: 10.1103/PhysRevLett.110.143603 PACS numbers: 42.50.Tx, 42.50.Wk, 79.20.Ds, 79.20.Eb Light that has a helical wave front due to an azimuthal phase shift, expðiL Þ (where L is an integer known as the topological charge), carries orbital angular momentum, L@. Such light is referred as an optical vortex [1][2][3][4]. Optical vortices have been widely investigated for applications such as optical trapping and guiding [5][6][7], as well as superresolution microscopy [8,9]. Circularly polarized light has a helical electric field and a spin angular momentum, S@, associated with its circular polarization. Optical vortices with circular polarization exhibit both wave front and polarization helicities, and a total angular momentum, J@ [10-12], which is defined as the sum of the orbital and spin angular momenta. This angular momentum is evidenced by the orbital and spinning motions of trapped particles in optical tweezers.To date, several researchers have intensely studied the interaction of structured light, such as radially polarized beams, with plasmonic or metallic structures [13][14][15]. However, these previous studies mostly focused on optical properties, such as mode selection, plasmon focusing, etc., of plasmonic or metallic structures, including photonic crystals as well as plasmonic waveguides, prepared by conventional integrated photonic circuit techniques based on lithography and chemical etching. There are few reports on the use of structured light itself to form chiral structures on the nanoscale. Recently, we discovered that the helicity of a circularly polarized optical vortex can be directly transferred to an irradiated metal sample, resulting in the formation of chiral nanoneedles [16][17][18]. This is the first demonstration, to the best of our knowledge, of nanostructures created by structured light with angular momenta, and it clearly represents a new scientific phenomenon.We have also investigated control of the chirality of formed nanoneedles by changing the sign of the optical vortex helicity. Chiral nanostructures have the potential to form many new material structures [19], including planar chiral metamaterials [20,21] and plasmonic nanostructures [22,23]. They can also be used to selectively identify the chirality of chemical composites in nanoscale imaging systems, such as atomic force and scanning tunnel microscopes [24][25][26][27].However, it is currently unclear whe...
The formation of a monocrystalline silicon needle by picosecond optical vortex pulse illumination was demonstrated for the first time in this study. The dynamics of this silicon needle formation was further revealed by employing an ultrahigh-speed camera. The melted silicon was collected through picosecond pulse deposition to the dark core of the optical vortex, forming the silicon needle on a submicrosecond time scale. The needle was composed of monocrystalline silicon with the same lattice index (100) as that of the silicon substrate, and had a height of approximately 14 μm and a thickness of approximately 3 μm. Overlaid vortex pulses allowed the needle to be shaped with a height of approximately 40 μm without any changes to the crystalline properties. Such a monocrystalline silicon needle can be applied to devices in many fields, such as core–shell structures for silicon photonics and photovoltaic devices as well as nano- or microelectromechanical systems.
Dietary Pi and parathyroid hormone (PTH) are two most important physiological and pathophysiological regulators of Pi re-absorption in the renal proximal tubule. Effects of dietary Pi on Na+/Pi co-transporter NaPi-2 were investigated in thyroparathyroidectomized (TPTX) rats. NaPi-2 protein and mRNA in the kidney cortex of TPTX rats were increased approximately 3.8- and 2.4-fold in amount respectively compared with those in the sham-operated animals. Administration of PTH to the TPTX rats resulted in a decrease in the amount of NaPi-2 protein, but not in the abundance of NaPi-2 mRNA. Deprivation of dietary Pi in the TPTX rats did not affect the amount of NaPi-2 mRNA and protein. In the Pi-deprived TPTX rats, feeding of a high-Pi diet resulted in marked decreases in Pi transport activity and the amount of NaPi-2 protein in the superficial nephrons. Immunohistochemical analysis demonstrated that administration of PTH to TPTX rats resulted in a decrease in NaPi-2 immunoreactivity from both superficial and juxtamedullary nephrons within 4 h. Switching TPTX animals from a low-Pi diet to the high-Pi diet decreased NaPi-2 immunoreactivity from superficial nephrons, but not from juxtamedullary nephrons, within 4 h. These results suggest that dietary Pi could regulate the amount of NaPi-2 protein in the superficial nephrons in a PTH-independent manner.
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